The two-dimensional freezing transition is very different from its three-dimensional counterpart. In contrast, the glass transition is usually assumed to have similar characteristics in two and three dimensions. Using computer simulations, here we show that glassy dynamics in supercooled two- and three-dimensional fluids are fundamentally different. Specifically, transient localization of particles on approaching the glass transition is absent in two dimensions, whereas it is very pronounced in three dimensions. Moreover, the temperature dependence of the relaxation time of orientational correlations is decoupled from that of the translational relaxation time in two dimensions but not in three dimensions. Last, the relationships between the characteristic size of dynamically heterogeneous regions and the relaxation time are very different in two and three dimensions. These results strongly suggest that the glass transition in two dimensions is different than in three dimensions.
机构:
Mokpo Natl Maritime Univ, Div Liberal Arts & Sci, Mokpo 530729, South KoreaMokpo Natl Maritime Univ, Div Liberal Arts & Sci, Mokpo 530729, South Korea
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Princeton Univ, Lewis Sigler Inst, Carl Icahn Lab 170, Princeton, NJ 08544 USA
Univ Calif San Diego, Dept Phys, La Jolla, CA 92093 USA
Univ Calif San Diego, Dept Biol, La Jolla, CA 92093 USAPrinceton Univ, Lewis Sigler Inst, Carl Icahn Lab 170, Princeton, NJ 08544 USA
Schoetz, Eva-Maria
Lanio, Marcos
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Princeton Univ, Lewis Sigler Inst, Carl Icahn Lab 170, Princeton, NJ 08544 USAPrinceton Univ, Lewis Sigler Inst, Carl Icahn Lab 170, Princeton, NJ 08544 USA
Lanio, Marcos
Talbot, Jared A.
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Princeton Univ, Lewis Sigler Inst, Carl Icahn Lab 170, Princeton, NJ 08544 USAPrinceton Univ, Lewis Sigler Inst, Carl Icahn Lab 170, Princeton, NJ 08544 USA
Talbot, Jared A.
Manning, M. Lisa
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Syracuse Univ, Dept Phys, Syracuse, NY 13244 USAPrinceton Univ, Lewis Sigler Inst, Carl Icahn Lab 170, Princeton, NJ 08544 USA