Applications of adsorption microcalorimetry for the characterization of metal-based catalysts

被引：26

作者：

Spiewak, BE ^{[1
]}

Dumesic, JA ^{[1
]}

机构：

[1] Univ Wisconsin, Dept Chem Engn, Madison, WI 53706 USA

来源：

THERMOCHIMICA ACTA | 1998年 / 312卷 / 1-2期

基金：

美国国家科学基金会;

关键词：

adsorption; catalysts; microcalorimetry; powders; single crystals; thin films; transition metals;

D O I：

10.1016/S0040-6031(97)00443-7

中图分类号：

O414.1 [热力学];

学科分类号：

摘要：

Microcalorimetry is a useful tool for studies of heterogeneous catalysts, because it provides a direct measurement of the strength with which molecules interact with solid surfaces. The following communication reviews adsorption microcalorimetric studies of unsupported metals and metal-based catalysts performed over the last 20 years, and then presents three advanced microcalorimetric techniques and their applications to the study of low surface-area-metal single crystals, films and powders, and metal surfaces/catalysts that are highly reactive toward oxygenates. (C) 1998 Elsevier Science B.V.

引用

页码：95 / 104

页数：10

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