Energy consumption and optimal reactor configuration for nonthermal plasma conversion of N2O in nitrogen and N2O in argon

被引:17
|
作者
Zhao, GB
Hu, XD
Plumb, OA
Radosz, M [1 ]
机构
[1] Univ Wyoming, Dept Chem & Petr Engn, Laramie, WY 82071 USA
[2] Univ Wyoming, Coll Engn, Laramie, WY 82071 USA
关键词
D O I
10.1021/ef049966c
中图分类号
TE [石油、天然气工业]; TK [能源与动力工程];
学科分类号
0807 ; 0820 ;
摘要
The analysis of experimental data, chemical reaction mechanisms, and kinetic modeling data is used to determine the power input and pulsed-corona-discharge reactor configuration that minimizes energy consumption for converting N2O in nitrogen and N2O in argon, which are model binaries reminiscent of more complex NOx in flue gas systems. Specifically, it is found that inseries reactors are much more energy efficient than a single reactor and more energy efficient than parallel reactors. For example, 12 reactors in series are needed to remove 90% of N2O if its initial concentration in nitrogen is about 200 ppm.
引用
收藏
页码:1522 / 1530
页数:9
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