Energy consumption and optimal reactor configuration for nonthermal plasma conversion of N2O in nitrogen and N2O in argon

被引:17
|
作者
Zhao, GB
Hu, XD
Plumb, OA
Radosz, M [1 ]
机构
[1] Univ Wyoming, Dept Chem & Petr Engn, Laramie, WY 82071 USA
[2] Univ Wyoming, Coll Engn, Laramie, WY 82071 USA
关键词
D O I
10.1021/ef049966c
中图分类号
TE [石油、天然气工业]; TK [能源与动力工程];
学科分类号
0807 ; 0820 ;
摘要
The analysis of experimental data, chemical reaction mechanisms, and kinetic modeling data is used to determine the power input and pulsed-corona-discharge reactor configuration that minimizes energy consumption for converting N2O in nitrogen and N2O in argon, which are model binaries reminiscent of more complex NOx in flue gas systems. Specifically, it is found that inseries reactors are much more energy efficient than a single reactor and more energy efficient than parallel reactors. For example, 12 reactors in series are needed to remove 90% of N2O if its initial concentration in nitrogen is about 200 ppm.
引用
收藏
页码:1522 / 1530
页数:9
相关论文
共 50 条
  • [21] Nitrogen removal with energy recovery through N2O decomposition
    Scherson, Yaniv D.
    Wells, George F.
    Woo, Sung-Geun
    Lee, Jangho
    Park, Joonhong
    Cantwell, Brian J.
    Criddle, Craig S.
    ENERGY & ENVIRONMENTAL SCIENCE, 2013, 6 (01) : 241 - 248
  • [22] Conversion of N2O in gliding arc discharges
    Krawczyk, K
    Mlotek, M
    Rzepecka, K
    PRZEMYSL CHEMICZNY, 2003, 82 (10): : 1387 - 1390
  • [23] Conversion of NO to N2O on MgO thin films
    Di Valentin, C
    Pacchioni, G
    Abbet, S
    Heiz, U
    JOURNAL OF PHYSICAL CHEMISTRY B, 2002, 106 (31): : 7666 - 7673
  • [24] Velocity of N2 upon dissociation of N2O in N2O•(H2O)m
    Gandhi, SR
    JOURNAL OF PHYSICAL CHEMISTRY A, 1999, 103 (50): : 10713 - 10718
  • [25] Biochar mitigates the stimulatory effects of straw incorporation on N2O emission and N2O/(N2O + N2) ratio in upland soil
    Li, Chenglin
    Wei, Zhijun
    Wang, Xiaomin
    Ma, Xiaofang
    Tang, Quan
    Zhao, Bingzi
    Shan, Jun
    Yan, Xiaoyuan
    JOURNAL OF ENVIRONMENTAL MANAGEMENT, 2024, 369
  • [26] EXPOSURE TO N2O
    FANCOURTSMITH, PF
    KAPNOUDHIS, P
    BRAND, SC
    CANADIAN JOURNAL OF ANAESTHESIA-JOURNAL CANADIEN D ANESTHESIE, 1993, 40 (04): : 396 - 397
  • [27] N2O emission and the N2O/(N2O + N2) product ratio of denitrification as controlled by available carbon substrates and nitrate concentrations
    Senbayram, M.
    Chen, R.
    Budai, A.
    Bakken, L.
    Dittert, K.
    AGRICULTURE ECOSYSTEMS & ENVIRONMENT, 2012, 147 : 4 - 12
  • [28] N2O revalorization
    Chen J.-J.
    Huang H.-M.
    Nature Chemistry, 2022, 14 (8) : 846 - 848
  • [29] N2O emission dynamics along an intertidal elevation gradient in a subtropical estuary: Importance of N2O consumption
    Gao, Dengzhou
    Hou, Lijun
    Liu, Min
    Zheng, Yanling
    Yin, Guoyu
    Niu, Yuhui
    ENVIRONMENTAL RESEARCH, 2022, 205
  • [30] Global N2O balance and nitrogen fertilizer
    Kawashima, H
    Bazin, MJ
    Lynch, JM
    ECOLOGICAL MODELLING, 1996, 87 (1-3) : 51 - 57