Robust evidence for reversal of the trend in aerosol effective climate forcing

被引:56
|
作者
Quaas, Johannes [1 ]
Jia, Hailing [1 ]
Smith, Chris [2 ,3 ]
Albright, Anna Lea [4 ]
Aas, Wenche [5 ]
Bellouin, Nicolas [6 ,7 ]
Boucher, Olivier [6 ]
Doutriaux-Boucher, Marie [8 ]
Forster, Piers M. [2 ]
Grosvenor, Daniel [2 ]
Jenkins, Stuart [9 ]
Klimont, Zbigniew [3 ]
Loeb, Norman G. [10 ]
Ma, Xiaoyan [11 ]
Naik, Vaishali [12 ]
Paulot, Fabien [12 ]
Stier, Philip [9 ]
Wild, Martin [13 ]
Myhre, Gunnar [14 ]
Schulz, Michael [15 ]
机构
[1] Univ Leipzig, Inst Meteorol, Leipzig, Germany
[2] Univ Leeds, Sch Earth & Environm, Leeds, W Yorkshire, England
[3] Int Inst Appl Syst Anal, Laxenburg, Austria
[4] Sorbonne Univ, Inst Pierre Simon Laplace, Lab Meteorol Dynam, Paris, France
[5] Norwegian Inst Air Res, Kjeller, Norway
[6] Sorbonne Univ, Inst Pierre Simon Laplace, CNRS, Paris, France
[7] Univ Reading, Dept Meteorol, Reading, Berks, England
[8] EUMETSAT, Darmstadt, Germany
[9] Univ Oxford, Atmospher Ocean & Planetary Phys, Oxford, England
[10] NASA, Langley Res Ctr, Hampton, VA 23665 USA
[11] Nanjing Univ Informat Sci & Technol, Sch Atmospher Phys, Nanjing, Peoples R China
[12] Geophys Fluid Dynam Lab, Princeton, NJ USA
[13] Swiss Fed Inst Technol, Dept Environm Syst Sci, Zurich, Switzerland
[14] CICERO, Oslo, Norway
[15] Norwegian Meteorol Inst, Oslo, Norway
基金
欧盟地平线“2020”;
关键词
SOLAR-RADIATION RECORDS; EARTH SYSTEM MODEL; OPTICAL DEPTH; CLOUD INTERACTIONS; SATELLITE-OBSERVATIONS; DROPLET NUMBER; AIR-POLLUTION; ANTHROPOGENIC EMISSIONS; CLEAR-SKY; DECADES;
D O I
10.5194/acp-22-12221-2022
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Anthropogenic aerosols exert a cooling influence that offsets part of the greenhouse gas warming. Due to their short tropospheric lifetime of only several days, the aerosol forcing responds quickly to emissions. Here, we present and discuss the evolution of the aerosol forcing since 2000. There are multiple lines of evidence that allow us to robustly conclude that the anthropogenic aerosol effective radiative forcing (ERF) - both aerosol- radiation interactions (ERFari) and aerosol-cloud interactions (ERFaci) - has become less negative globally, i.e. the trend in aerosol effective radiative forcing changed sign from negative to positive. Bottom-up inventories show that anthropogenic primary aerosol and aerosol precursor emissions declined in most regions of the world; observations related to aerosol burden show declining trends, in particular of the fine-mode particles that make up most of the anthropogenic aerosols; satellite retrievals of cloud droplet numbers show trends in regions with aerosol declines that are consistent with these in sign, as do observations of top-of-atmosphere radiation. Climate model results, including a revised set that is constrained by observations of the ocean heat content evolution show a consistent sign and magnitude for a positive forcing relative to the year 2000 due to reduced aerosol effects. This reduction leads to an acceleration of the forcing of climate change, i.e. an increase in forcing by 0.1 to 0.3 W m(-2), up to 12 % of the total climate forcing in 2019 compared to 1750 according to the Intergovernmental Panel on Climate Change (IPCC).
引用
收藏
页码:12221 / 12239
页数:19
相关论文
共 50 条
  • [41] Greenhouse-gas versus aerosol forcing and African climate response
    Paeth, H
    Feichter, J
    CLIMATE DYNAMICS, 2006, 26 (01) : 35 - 54
  • [42] Inferred Net Aerosol Forcing Based on Historical Climate Changes: a Review
    Chris E. Forest
    Current Climate Change Reports, 2018, 4 : 11 - 22
  • [43] Energy Budget Constraints on the Time History of Aerosol Forcing and Climate Sensitivity
    Smith, C. J.
    Harris, G. R.
    Palmer, M. D.
    Bellouin, N.
    Collins, W.
    Myhre, G.
    Schulz, M.
    Golaz, J. -C.
    Ringer, M.
    Storelvmo, T.
    Forster, P. M.
    JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2021, 126 (13)
  • [44] Monitoring of aerosol forcing of climate from space: analysis of measurement requirements
    Mishchenko, MI
    Cairns, B
    Hansen, JE
    Travis, LD
    Burg, R
    Kaufman, YJ
    Martins, JV
    Shettle, EP
    JOURNAL OF QUANTITATIVE SPECTROSCOPY & RADIATIVE TRANSFER, 2004, 88 (1-3): : 149 - 161
  • [45] Satellite-based estimate of the direct and indirect aerosol climate forcing
    Quaas, Johannes
    Boucher, Olivier
    Bellouin, Nicolas
    Kinne, Stefan
    JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2008, 113 (D5)
  • [46] Simulation of aerosol distributions and radiative forcing for INDOEX: Regional climate impacts
    Collins, WD
    Rasch, PJ
    Eaton, BE
    Fillmore, DW
    Kiehl, JT
    Beck, CT
    Zender, CS
    JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2002, 107 (D19)
  • [47] Indirect sulphate aerosol forcing in a climate model with an interactive sulphur cycle
    Jones, A
    Roberts, DL
    Woodage, MJ
    Johnson, CE
    JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2001, 106 (D17) : 20293 - 20310
  • [48] Greenhouse-gas versus aerosol forcing and African climate response
    Heiko Paeth
    Johann Feichter
    Climate Dynamics, 2006, 26 : 35 - 54
  • [49] Aerosol and ozone changes as forcing for climate evolution between 1850 and 2100
    Szopa, Sophie
    Balkanski, Y.
    Schulz, M.
    Bekki, S.
    Cugnet, D.
    Fortems-Cheiney, A.
    Turquety, S.
    Cozic, A.
    Deandreis, C.
    Hauglustaine, D.
    Idelkadi, A.
    Lathiere, J.
    Lefevre, F.
    Marchand, M.
    Vuolo, R.
    Yan, N.
    Dufresne, J-L.
    CLIMATE DYNAMICS, 2013, 40 (9-10) : 2223 - 2250
  • [50] The impact of humidity above stratiform clouds on indirect aerosol climate forcing
    Andrew S. Ackerman
    Michael P. Kirkpatrick
    David E. Stevens
    Owen B. Toon
    Nature, 2004, 432 : 1014 - 1017