Robust evidence for reversal of the trend in aerosol effective climate forcing

被引:56
|
作者
Quaas, Johannes [1 ]
Jia, Hailing [1 ]
Smith, Chris [2 ,3 ]
Albright, Anna Lea [4 ]
Aas, Wenche [5 ]
Bellouin, Nicolas [6 ,7 ]
Boucher, Olivier [6 ]
Doutriaux-Boucher, Marie [8 ]
Forster, Piers M. [2 ]
Grosvenor, Daniel [2 ]
Jenkins, Stuart [9 ]
Klimont, Zbigniew [3 ]
Loeb, Norman G. [10 ]
Ma, Xiaoyan [11 ]
Naik, Vaishali [12 ]
Paulot, Fabien [12 ]
Stier, Philip [9 ]
Wild, Martin [13 ]
Myhre, Gunnar [14 ]
Schulz, Michael [15 ]
机构
[1] Univ Leipzig, Inst Meteorol, Leipzig, Germany
[2] Univ Leeds, Sch Earth & Environm, Leeds, W Yorkshire, England
[3] Int Inst Appl Syst Anal, Laxenburg, Austria
[4] Sorbonne Univ, Inst Pierre Simon Laplace, Lab Meteorol Dynam, Paris, France
[5] Norwegian Inst Air Res, Kjeller, Norway
[6] Sorbonne Univ, Inst Pierre Simon Laplace, CNRS, Paris, France
[7] Univ Reading, Dept Meteorol, Reading, Berks, England
[8] EUMETSAT, Darmstadt, Germany
[9] Univ Oxford, Atmospher Ocean & Planetary Phys, Oxford, England
[10] NASA, Langley Res Ctr, Hampton, VA 23665 USA
[11] Nanjing Univ Informat Sci & Technol, Sch Atmospher Phys, Nanjing, Peoples R China
[12] Geophys Fluid Dynam Lab, Princeton, NJ USA
[13] Swiss Fed Inst Technol, Dept Environm Syst Sci, Zurich, Switzerland
[14] CICERO, Oslo, Norway
[15] Norwegian Meteorol Inst, Oslo, Norway
基金
欧盟地平线“2020”;
关键词
SOLAR-RADIATION RECORDS; EARTH SYSTEM MODEL; OPTICAL DEPTH; CLOUD INTERACTIONS; SATELLITE-OBSERVATIONS; DROPLET NUMBER; AIR-POLLUTION; ANTHROPOGENIC EMISSIONS; CLEAR-SKY; DECADES;
D O I
10.5194/acp-22-12221-2022
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Anthropogenic aerosols exert a cooling influence that offsets part of the greenhouse gas warming. Due to their short tropospheric lifetime of only several days, the aerosol forcing responds quickly to emissions. Here, we present and discuss the evolution of the aerosol forcing since 2000. There are multiple lines of evidence that allow us to robustly conclude that the anthropogenic aerosol effective radiative forcing (ERF) - both aerosol- radiation interactions (ERFari) and aerosol-cloud interactions (ERFaci) - has become less negative globally, i.e. the trend in aerosol effective radiative forcing changed sign from negative to positive. Bottom-up inventories show that anthropogenic primary aerosol and aerosol precursor emissions declined in most regions of the world; observations related to aerosol burden show declining trends, in particular of the fine-mode particles that make up most of the anthropogenic aerosols; satellite retrievals of cloud droplet numbers show trends in regions with aerosol declines that are consistent with these in sign, as do observations of top-of-atmosphere radiation. Climate model results, including a revised set that is constrained by observations of the ocean heat content evolution show a consistent sign and magnitude for a positive forcing relative to the year 2000 due to reduced aerosol effects. This reduction leads to an acceleration of the forcing of climate change, i.e. an increase in forcing by 0.1 to 0.3 W m(-2), up to 12 % of the total climate forcing in 2019 compared to 1750 according to the Intergovernmental Panel on Climate Change (IPCC).
引用
收藏
页码:12221 / 12239
页数:19
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