Robust evidence for reversal of the trend in aerosol effective climate forcing

被引:56
|
作者
Quaas, Johannes [1 ]
Jia, Hailing [1 ]
Smith, Chris [2 ,3 ]
Albright, Anna Lea [4 ]
Aas, Wenche [5 ]
Bellouin, Nicolas [6 ,7 ]
Boucher, Olivier [6 ]
Doutriaux-Boucher, Marie [8 ]
Forster, Piers M. [2 ]
Grosvenor, Daniel [2 ]
Jenkins, Stuart [9 ]
Klimont, Zbigniew [3 ]
Loeb, Norman G. [10 ]
Ma, Xiaoyan [11 ]
Naik, Vaishali [12 ]
Paulot, Fabien [12 ]
Stier, Philip [9 ]
Wild, Martin [13 ]
Myhre, Gunnar [14 ]
Schulz, Michael [15 ]
机构
[1] Univ Leipzig, Inst Meteorol, Leipzig, Germany
[2] Univ Leeds, Sch Earth & Environm, Leeds, W Yorkshire, England
[3] Int Inst Appl Syst Anal, Laxenburg, Austria
[4] Sorbonne Univ, Inst Pierre Simon Laplace, Lab Meteorol Dynam, Paris, France
[5] Norwegian Inst Air Res, Kjeller, Norway
[6] Sorbonne Univ, Inst Pierre Simon Laplace, CNRS, Paris, France
[7] Univ Reading, Dept Meteorol, Reading, Berks, England
[8] EUMETSAT, Darmstadt, Germany
[9] Univ Oxford, Atmospher Ocean & Planetary Phys, Oxford, England
[10] NASA, Langley Res Ctr, Hampton, VA 23665 USA
[11] Nanjing Univ Informat Sci & Technol, Sch Atmospher Phys, Nanjing, Peoples R China
[12] Geophys Fluid Dynam Lab, Princeton, NJ USA
[13] Swiss Fed Inst Technol, Dept Environm Syst Sci, Zurich, Switzerland
[14] CICERO, Oslo, Norway
[15] Norwegian Meteorol Inst, Oslo, Norway
基金
欧盟地平线“2020”;
关键词
SOLAR-RADIATION RECORDS; EARTH SYSTEM MODEL; OPTICAL DEPTH; CLOUD INTERACTIONS; SATELLITE-OBSERVATIONS; DROPLET NUMBER; AIR-POLLUTION; ANTHROPOGENIC EMISSIONS; CLEAR-SKY; DECADES;
D O I
10.5194/acp-22-12221-2022
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Anthropogenic aerosols exert a cooling influence that offsets part of the greenhouse gas warming. Due to their short tropospheric lifetime of only several days, the aerosol forcing responds quickly to emissions. Here, we present and discuss the evolution of the aerosol forcing since 2000. There are multiple lines of evidence that allow us to robustly conclude that the anthropogenic aerosol effective radiative forcing (ERF) - both aerosol- radiation interactions (ERFari) and aerosol-cloud interactions (ERFaci) - has become less negative globally, i.e. the trend in aerosol effective radiative forcing changed sign from negative to positive. Bottom-up inventories show that anthropogenic primary aerosol and aerosol precursor emissions declined in most regions of the world; observations related to aerosol burden show declining trends, in particular of the fine-mode particles that make up most of the anthropogenic aerosols; satellite retrievals of cloud droplet numbers show trends in regions with aerosol declines that are consistent with these in sign, as do observations of top-of-atmosphere radiation. Climate model results, including a revised set that is constrained by observations of the ocean heat content evolution show a consistent sign and magnitude for a positive forcing relative to the year 2000 due to reduced aerosol effects. This reduction leads to an acceleration of the forcing of climate change, i.e. an increase in forcing by 0.1 to 0.3 W m(-2), up to 12 % of the total climate forcing in 2019 compared to 1750 according to the Intergovernmental Panel on Climate Change (IPCC).
引用
收藏
页码:12221 / 12239
页数:19
相关论文
共 50 条
  • [1] Robust observational constraint of uncertain aerosol processes and emissions in a climate model and the effect on aerosol radiative forcing
    Johnson, Jill S.
    Regayre, Leighton A.
    Yoshioka, Masaru
    Pringle, Kirsty J.
    Turnock, Steven T.
    Browse, Jo
    Sexton, David M. H.
    Rostron, John W.
    Schutgens, Nick A. J.
    Partridge, Daniel G.
    Liu, Dantong
    Allan, James D.
    Coe, Hugh
    Ding, Aijun
    Cohen, David D.
    Atanacio, Armand
    Vakkari, Ville
    Asmi, Eija
    Carslaw, Ken S.
    ATMOSPHERIC CHEMISTRY AND PHYSICS, 2020, 20 (15) : 9491 - 9524
  • [2] Indirect aerosol forcing, quasi forcing, and climate response
    Rotstayn, LD
    Penner, JE
    JOURNAL OF CLIMATE, 2001, 14 (13) : 2960 - 2975
  • [3] Trend in atmospheric angular momentum in a transient climate change simulation with greenhouse gas and aerosol forcing
    Huang, HP
    Weickmann, KM
    Hsu, CJ
    JOURNAL OF CLIMATE, 2001, 14 (07) : 1525 - 1534
  • [4] Climate response to anthropogenic aerosol forcing
    Wang, Chien
    ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY, 2016, 252
  • [6] Interactive nature of climate change and aerosol forcing
    Nazarenko, L.
    Rind, D.
    Tsigaridis, K.
    Del Genio, A. D.
    Kelley, M.
    Tausnev, N.
    JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2017, 122 (06) : 3457 - 3480
  • [7] Constraining the Aerosol Radiative Forcing and Climate Sensitivity
    L. D. Danny Harvey
    Climatic Change, 2000, 44 : 413 - 418
  • [8] Constraining the aerosol radiative forcing and climate sensitivity
    Harvey, LDD
    CLIMATIC CHANGE, 2000, 44 (04) : 413 - 418
  • [9] Aerosol Effective Radiative Forcing in the Online Aerosol Coupled CAS-FGOALS-f3-L Climate Model
    Wang, Hao
    Dai, Tie
    Zhao, Min
    Goto, Daisuke
    Bao, Qing
    Takemura, Toshihiko
    Nakajima, Teruyuki
    Shi, Guangyu
    ATMOSPHERE, 2020, 11 (10)
  • [10] Some considerations in the aerosol forcing of climate.
    Seinfeld, JH
    ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY, 1997, 213 : 79 - ENVR