atmospheric omission;
anthropogenic sources;
mercury and its species;
D O I:
10.1016/S1352-2310(01)00102-9
中图分类号:
X [环境科学、安全科学];
学科分类号:
08 ;
0830 ;
摘要:
Estimates of atmospheric emissions of mercury from anthropogenic sources in Europe in 1995 are presented with the information on emissions of both total mercury and its major chemical and physical forms. The 1995 anthropogenic emissions of total emissions were estimated to be about 342 tonnes, a decrease of 45% compared to these emissions in 1990. Combustion of fuels, particularly coal has been the major source of anthropogenic emissions contributing to more than half to the total emissions. The emissions from coal combustion have not changed significantly over the past decade. Major decrease has been estimated for emissions from industrial processes, particularly the chlor-alkali production using the Hg cell process. In 1995 the Europe emissions of anthropogenic mercury contributed about 13% to the global emissions of this element from anthropogenic sources. The anthropogenic Hg emissions in Europe were still higher than the natural emissions in the region, estimated to be about 250-300 tonnes per year. The accuracy of estimates of anthropogenic emissions of Hg in Europe in 1995 is considered to be between 25 and 50%. The most accurate seem to be the estimates for combustion sources, while the most incomplete data were collected and/or estimated for waste disposal. The emissions of gaseous elemental mercury contributed about 61% to the emissions of the total mercury, while the contribution of gaseous bivalent mercury and particulate mercury was 32 and 7%, respectively. (C) 2001 Elsevier Science Ltd. All rights reserved.
机构:
State Key Laboratory of Environmental Geochemistry,Institute of Geochemistry, Chinese Academy of Sciences
University of Chinese Academy of SciencesState Key Laboratory of Environmental Geochemistry,Institute of Geochemistry, Chinese Academy of Sciences
Xiaohang Xu
Na Liu
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机构:
State Key Laboratory of Environmental Geochemistry,Institute of Geochemistry, Chinese Academy of SciencesState Key Laboratory of Environmental Geochemistry,Institute of Geochemistry, Chinese Academy of Sciences
Na Liu
Matthew S.Landis
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机构:
US EPA, Of?ce of Research and Development, Research Triangle ParkState Key Laboratory of Environmental Geochemistry,Institute of Geochemistry, Chinese Academy of Sciences
Matthew S.Landis
Xinbin Feng
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机构:
State Key Laboratory of Environmental Geochemistry,Institute of Geochemistry, Chinese Academy of SciencesState Key Laboratory of Environmental Geochemistry,Institute of Geochemistry, Chinese Academy of Sciences
Xinbin Feng
Guangle Qiu
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机构:
State Key Laboratory of Environmental Geochemistry,Institute of Geochemistry, Chinese Academy of SciencesState Key Laboratory of Environmental Geochemistry,Institute of Geochemistry, Chinese Academy of Sciences
机构:
State Key Laboratory of Environmental Geochemistry, Institute of Geochemistry, Chinese Academy of Sciences, Guiyang
University of Chinese Academy of Sciences, BeijingState Key Laboratory of Environmental Geochemistry, Institute of Geochemistry, Chinese Academy of Sciences, Guiyang
Xu X.
Liu N.
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机构:
State Key Laboratory of Environmental Geochemistry, Institute of Geochemistry, Chinese Academy of Sciences, GuiyangState Key Laboratory of Environmental Geochemistry, Institute of Geochemistry, Chinese Academy of Sciences, Guiyang
Liu N.
Landis M.S.
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机构:
US EPA, Office of Research and Development, Research Triangle Park, Durham, 27709, NCState Key Laboratory of Environmental Geochemistry, Institute of Geochemistry, Chinese Academy of Sciences, Guiyang
Landis M.S.
Feng X.
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机构:
State Key Laboratory of Environmental Geochemistry, Institute of Geochemistry, Chinese Academy of Sciences, GuiyangState Key Laboratory of Environmental Geochemistry, Institute of Geochemistry, Chinese Academy of Sciences, Guiyang
Feng X.
Qiu G.
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机构:
State Key Laboratory of Environmental Geochemistry, Institute of Geochemistry, Chinese Academy of Sciences, GuiyangState Key Laboratory of Environmental Geochemistry, Institute of Geochemistry, Chinese Academy of Sciences, Guiyang
机构:
Harvard Univ, John A Paulson Sch Engn & Appl Sci, Cambridge, MA 02138 USAHarvard Univ, John A Paulson Sch Engn & Appl Sci, Cambridge, MA 02138 USA
Zhang, Yanxu
Jacob, Daniel J.
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Harvard Univ, John A Paulson Sch Engn & Appl Sci, Cambridge, MA 02138 USA
Harvard Univ, Dept Earth & Planetary Sci, Cambridge, MA 02138 USAHarvard Univ, John A Paulson Sch Engn & Appl Sci, Cambridge, MA 02138 USA
Jacob, Daniel J.
Horowitz, Hannah M.
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Harvard Univ, John A Paulson Sch Engn & Appl Sci, Cambridge, MA 02138 USAHarvard Univ, John A Paulson Sch Engn & Appl Sci, Cambridge, MA 02138 USA
Horowitz, Hannah M.
Chen, Long
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机构:
Harvard Univ, John A Paulson Sch Engn & Appl Sci, Cambridge, MA 02138 USA
Peking Univ, Coll Urban & Environm Sci, Beijing 100871, Peoples R ChinaHarvard Univ, John A Paulson Sch Engn & Appl Sci, Cambridge, MA 02138 USA
Chen, Long
Amos, Helen M.
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Harvard Univ, John A Paulson Sch Engn & Appl Sci, Cambridge, MA 02138 USAHarvard Univ, John A Paulson Sch Engn & Appl Sci, Cambridge, MA 02138 USA
Amos, Helen M.
Krabbenhoft, David P.
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机构:
US Geol Survey, Wisconsin Water Sci Ctr, Middleton, WI 53562 USAHarvard Univ, John A Paulson Sch Engn & Appl Sci, Cambridge, MA 02138 USA
Krabbenhoft, David P.
Slemr, Franz
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机构:
Max Planck Inst Chem, Dept Atmospher Chem, D-55128 Mainz, GermanyHarvard Univ, John A Paulson Sch Engn & Appl Sci, Cambridge, MA 02138 USA
Slemr, Franz
St Louis, Vincent L.
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机构:
Univ Alberta, Dept Biol Sci, Edmonton, AB T6G 2R3, CanadaHarvard Univ, John A Paulson Sch Engn & Appl Sci, Cambridge, MA 02138 USA
St Louis, Vincent L.
Sunderland, Elsie M.
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机构:
Harvard Univ, John A Paulson Sch Engn & Appl Sci, Cambridge, MA 02138 USA
Harvard Univ, Dept Environm Hlth, TH Chan Sch Publ Hlth, Boston, MA 02115 USAHarvard Univ, John A Paulson Sch Engn & Appl Sci, Cambridge, MA 02138 USA