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A Comprehensive Global Inventory of Atmospheric Antimony Emissions from Anthropogenic Activities, 1995-2010
被引:87
|作者:
Tian, Hezhong
[1
,3
]
Zhou, JunRui
[1
]
Zhu, Chuanyong
[1
]
Zhao, Dan
[1
]
Gao, Jiajia
[1
]
Hao, Jiming
[2
,3
]
He, Mengchang
[1
]
Liu, Kaiyun
[1
]
Wang, Kun
[1
]
Hua, Shenbing
[1
]
机构:
[1] Beijing Normal Univ, Sch Environm, State Key Joint Lab Environm Simulat & Pollut Con, Beijing 100875, Peoples R China
[2] Tsinghua Univ, Inst Environm Sci & Engn, Beijing 10084, Peoples R China
[3] State Environm Protect Key Lab Sources & Control, Beijing 100084, Peoples R China
基金:
中国国家自然科学基金;
关键词:
AIRBORNE PARTICULATE MATTER;
BRAKE ABRASION DUSTS;
TRACE-ELEMENTS;
COAL COMBUSTION;
HEAVY-METALS;
MERCURY;
AIR;
CONTAMINATION;
POLLUTANTS;
BEHAVIOR;
D O I:
10.1021/es405817u
中图分类号:
X [环境科学、安全科学];
学科分类号:
08 ;
0830 ;
摘要:
Antimony (Sb) and its compounds are considered as global pollutants due to their health risks and long-range transport characteristics. A comprehensive global inventory of atmospheric antimony emissions from anthropogenic activities during the period of 1995-2010 has been developed with specific estimation methods based on the relevant data available for different continents and countries. Our results indicate that the global antimony emissions have increased to a peak at about 2232 t (t) in 2005 and then declined gradually. Global antimony emissions in 2010 are estimated at about 1904 t (uncertainty of a 95% confidence interval (CI): -30% similar to 67%), with fuel combustion as the major source category. Asia and Europe account for about 57% and 24%, respectively, of the global total emissions, and China, the United States, and Japan rank as the top three emitting countries. Furthermore, global antimony emissions are distributed into gridded cells with a resolution of 1 degrees x 1 degrees. Regions with high Sb emissions are generally concentrated in the Southeastern Asia and Western Europe, while South Africa, economically developed regions in the eastern U.S., and Mexico are also responsible for the high antimony emission intensity.
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页码:10235 / 10241
页数:7
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