The Landau-Zener-Stuckelberg-Majorana transition in the T2 << T1 limit

被引:0
|
作者
Boucher, Michael C. [1 ]
Sun, Peter [1 ]
Keresztes, Ivan [1 ]
Harrell, Lee E. [2 ]
Marohn, John A. [1 ]
机构
[1] Cornell Univ, Dept Chem & Chem Biol, Ithaca, NY 14853 USA
[2] US Mil Acad, Dept Phys & Nucl Engn, West Point, NY 10996 USA
基金
美国国家卫生研究院;
关键词
Landau-Zener-Stuckelberg-Majorana transition; Landau-Zener transition; Bloch equations; Electron spin resonance; Saturation; Adiabatic rapid passage; Magnetic resonance force microscopy; Force-gradient detected magnetic resonance; NUCLEAR MAGNETIC-RELAXATION; ROTATING-FRAME RELAXATION; ADIABATIC PULSES; BROAD-BAND; BLOCH EQUATIONS; ELECTRON-SPIN; RESONANCE; INVERSION; DYNAMICS; CONVERGENCE;
D O I
10.1016/j.jmr.2023.107523
中图分类号
Q5 [生物化学];
学科分类号
071010 ; 081704 ;
摘要
Landau-Zener-Stuckelberg-Majorana (LZSM) transitions occur between quantum states when parameters in the system's Hamiltonian are varied continuously and rapidly. In magnetic resonance, losses in adiabatic rapid passage can be understood using the physics of LZSM transitions. Most treatments of LZSM transitions ignore the T-2 dephasing of coherences, however. Motivated by ongoing work in magnetic resonance force microscopy, we employ the Bloch equations, coordinate transformation, and the Magnus expansion to derive expressions for the final magnetization following a rapid field sweep at fixed irradiation intensity that include T-2 losses. Our derivation introduces an inversion-function, Fourier transform method for numerically evaluating highly oscillatory integrals. Expressions for the final magnetization are given for low and high irradiation intensity, valid in the T-2 << T-1 limit. Analytical results are compared to numerical simulations and nuclear magnetic resonance experiments. Our relatively straightforward calculation reproduces semiquantitatively the well known LZSM result in the T-2 -> 0 limit.
引用
收藏
页数:15
相关论文
共 50 条
  • [41] The Bloch equations when T1 = T2
    Rourke, David E.
    Karabanov, Alexander A.
    Booth, George H.
    Frantsuzov, Ilya
    INVERSE PROBLEMS, 2007, 23 (02) : 609 - 623
  • [42] Time related changes of T1, T2, and T2* of human blood in vitro
    Petrovic, Andreas
    Krauskopf, Astrid
    Hassler, Eva
    Stollberger, Rudolf
    Scheurer, Eva
    FORENSIC SCIENCE INTERNATIONAL, 2016, 262 : 11 - 17
  • [43] MRI Signal in Biological Tissues - Proton, Spin, T1, T2, T2☆
    Gorny, K.
    MEDICAL PHYSICS, 2016, 43 (06) : 3816 - 3816
  • [44] Simultaneous T1, T2, and T2*Mapping of Carotid Plaque: The SIMPLE* Technique
    Wang, Yajie
    Liu, Xiaoming
    Wang, Jing
    Wang, Yishi
    Qi, Haikun
    Kong, Xiangchuang
    Liu, Dingxi
    Liu, Jia
    Zheng, Hanpei
    Xiong, Fu
    Zhang, Lan
    Fu, Xiaona
    Zhang, Xinli
    Guo, Rui
    Qiao, Huiyu
    Chen, Zhensen
    Si, Dongyue
    Chen, Huijun
    RADIOLOGY, 2023, 307 (03)
  • [45] Free-breathing simultaneous T1, T2, and T2* quantification in the myocardium
    Hermann, Ingo
    Kellman, Peter
    Demirel, Omer B.
    Akcakaya, Mehmet
    Schad, Lothar R.
    Weingartner, Sebastian
    MAGNETIC RESONANCE IN MEDICINE, 2021,
  • [46] T1 and T2 measurements of the neonatal brain at 7 T
    Mahmoud, Aiman
    Tomi-Tricot, Raphael
    Leitao, David
    Bridgen, Philippa
    Price, Anthony N.
    Uus, Alena
    Boutillon, Arnaud
    Lawrence, Andrew J.
    Cromb, Daniel
    Cawley, Paul
    Deprez, Maria
    De Vita, Enrico
    Giles, Sharon L.
    Rutherford, Mary A.
    Edwards, A. David
    Hajnal, Joseph V.
    Arichi, Tomoki
    Malik, Shaihan J.
    MAGNETIC RESONANCE IN MEDICINE, 2025, 93 (05) : 2153 - 2162
  • [47] Visibility study of S-T+ Landau-Zener-Stuckelberg oscillations without applied initialization
    Granger, G.
    Aers, G. C.
    Studenikin, S. A.
    Kam, A.
    Zawadzki, P.
    Wasilewski, Z. R.
    Sachrajda, A. S.
    PHYSICAL REVIEW B, 2015, 91 (11):
  • [48] Reproducibility of myocardial T1 and T2 relaxation time measurement using slice-interleaved T1 and T2 mapping sequences
    Bellm, Steven
    Basha, Tamer A.
    Shah, Ravi V.
    Murthy, Venkatesh L.
    Liew, Charlene
    Tang, Maxine
    Ngo, Long H.
    Manning, Warren J.
    Nezafat, Reza
    JOURNAL OF MAGNETIC RESONANCE IMAGING, 2016, 44 (05) : 1159 - 1167
  • [49] MRI measurements of T1, T2 and D for gels undergoing volume phase transition
    Yung, KT
    MAGNETIC RESONANCE IMAGING, 2003, 21 (02) : 135 - 144
  • [50] SPLITTING OF ALPHA(T1 AND T2) AND RELATED QUESTIONS
    CONWAY, JB
    WU, PY
    NOTICES OF THE AMERICAN MATHEMATICAL SOCIETY, 1975, 22 (06): : A633 - A633