Reengineering the old wingmen: Increasing K+ coverage to boost electrocatalytic CO2RR on Cu

被引:1
|
作者
Hus, Matej [1 ,2 ,3 ]
Likozar, Blaz [1 ,4 ]
机构
[1] Natl Inst Chem, Hajdrihova 19, Ljubljana 1000, Slovenia
[2] Assoc Tech Culture Slovenia, Zaloska 65, Ljubljana 1000, Slovenia
[3] Inst Protect Cultural Heritage, Poljanska 40, Ljubljana 1000, Slovenia
[4] Fac Polymer Technol, Ozare 19, Slovenj Gradec 2830, Slovenia
来源
CHEM CATALYSIS | 2023年 / 3卷 / 05期
关键词
ELECTROCHEMICAL REDUCTION; CO;
D O I
10.1016/j.checat.2023.100611
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Despite extensive research into combating greenhouse gas emis-sions, electrocatalytic CO2 reduction remains plagued by meager rates and C1 product formation. In the April issue of Cell Reports Physical Science, Fan and colleagues report on a catalyst modifica-tion using a synergy effect of K+ to form multi-carbon products on copper.
引用
收藏
页数:3
相关论文
共 42 条
  • [21] Cu acting as Fe activity promoter in dual-atom Cu/Fe-NC catalyst in CO2RR to C1 products
    Wei, Xiaofei
    Wei, Shuxian
    Cao, Shoufu
    Hu, Yuying
    Zhou, Sainan
    Liu, Siyuan
    Wang, Zhaojie
    Lu, Xiaoqing
    APPLIED SURFACE SCIENCE, 2021, 564
  • [22] Enhanced Local CO Coverage on Cu Quantum Dots for Boosting Electrocatalytic CO2 Reduction to Ethylene
    Wang, Yan
    Wang, Jiarui
    Cai, Rui
    Zhang, Jianfang
    Xia, Shuai
    Li, Zeping
    Yu, Cuiping
    Wu, Jingjie
    Wang, Peng
    Wu, Yucheng
    ADVANCED FUNCTIONAL MATERIALS, 2024,
  • [23] In situ oxidative etching-enabled synthesis of hollow Cu2O nanocrystals for efficient CO2RR into C2+ products
    Zhang, Haifeng
    Qiao, Yan
    Wang, Yingying
    Zheng, Yiqun
    Huang, Hongwen
    SUSTAINABLE ENERGY & FUELS, 2022, 6 (21) : 4860 - 4865
  • [24] Introducing Cu2O (111) phase on Cu(OH)2 nanorods integrated Pd-cocatalyst for boosting acetone selectivity via photoelectrochemical CO2RR
    Uthirakumar, Periyayya
    Kim, Dasom
    Dao, Vandung
    Kai, Chen
    Yun, Changmin
    Jang, Youn Jeong
    Lee, In-Hwan
    ENVIRONMENTAL RESEARCH, 2025, 265
  • [25] Intimate atomic Cu-Ag interfaces for high CO2RR selectivity towards CH4 at low over potential
    Choi, Chungseok
    Cai, Jin
    Lee, Changsoo
    Lee, Hyuck Mo
    Xu, Mingjie
    Huang, Yu
    NANO RESEARCH, 2021, 14 (10) : 3497 - 3501
  • [26] Enhancement of CO2RR product formation on Cu-ZnO-based electrodes by varying ink formulation and post-treatment methods
    Jaster, Theresa
    Albers, Simon
    Leonhard, Armin
    Kraeenbring, Mena-Alexander
    Lohmann, Heiko
    Zeidler-Fandrich, Barbara
    Ozcan, Fatih
    Segets, Doris
    Apfel, Ulf-Peter
    JOURNAL OF PHYSICS-ENERGY, 2023, 5 (02):
  • [27] Intimate atomic Cu-Ag interfaces for high CO2RR selectivity towards CH4 at low over potential
    Chungseok Choi
    Jin Cai
    Changsoo Lee
    Hyuck Mo Lee
    Mingjie Xu
    Yu Huang
    Nano Research, 2021, 14 : 3497 - 3501
  • [28] Geometric Modulation of Local CO Flux in Ag@Cu2O Nanoreactors for Steering the CO2RR Pathway toward High-Efficacy Methane Production
    Xiong, Likun
    Zhang, Xiang
    Chen, Ling
    Deng, Zhao
    Han, Sheng
    Chen, Yufeng
    Zhong, Jun
    Sun, Hao
    Lian, Yuebin
    Yang, Baiyu
    Yuan, Xuzhou
    Yu, Hui
    Liu, Yu
    Yang, Xiaoqin
    Guo, Jun
    Rummeli, Mark H.
    Jiao, Yan
    Peng, Yang
    ADVANCED MATERIALS, 2021, 33 (32)
  • [29] Impact of Cu+ and Cu2+ species on the oxide-metal transition processes of CuxO foams during the CO2RR probed by operando Quick-XAS
    Blaseio, S.
    Dosche, C.
    Rahaman, M.
    Kiran, K.
    Dworzak, A.
    Mahrt, B.
    Broekmann, P.
    Dutta, A.
    Oezaslan, M.
    JOURNAL OF MATERIALS CHEMISTRY A, 2024, 12 (41) : 28177 - 28192
  • [30] Binder-free Cu/Cu2O/CuO/Pd nanorods photoelectrode for regulating the faradaic efficiency for acetaldehyde and acetate production during photoelectrochemical CO2RR by stabilizing the Cu2O phase
    Uthirakumar, Periyayya
    Lee, Yeji
    Son, Hoki
    Dao, Vandung
    Kim, Chi Yeop
    Lee, In-Hwan
    JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING, 2023, 11 (06):