Metalloporphyrinic metal-organic frameworks for enhanced photocatalytic degradation of a mustard gas simulant

被引：1

作者：

Quon, Alisa S. ^{[1
]}

Manriquez, Doroteo ^{[1
]}

Nguyen, Anna ^{[1
,7
]}

Papazyan, Edgar K. ^{[1
]}

Wijeratne, Pavithra ^{[1
]}

An, Lun ^{[2
]}

Qi, Long ^{[2
]}

Tang, Matthew J. ^{[1
]}

Ready, Austin D. ^{[3
]}

Farha, Omar K. ^{[4
,5
,6
]}

Liu, Yangyang ^{[1
]}

机构：

[1] Calif State Univ Los Angeles, Dept Chem & Biochem, 5151 State Univ Dr, Los Angeles, CA 90032 USA

[2] Iowa State Univ, US DOE Ames Natl Lab, Ames, IA 50011 USA

[3] Univ Calif Los Angeles, Dept Chem & Biochem, 607 Charles E Young Dr East, Los Angeles, CA 90095 USA

[4] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA

[5] Northwestern Univ, Int Inst Nanotechnol IIN, Evanston, IL 60208 USA

[6] Northwestern Univ, Dept Chem & Biol Engn, Evanston, IL 60208 USA

[7] Calif Univ Sci & Med, Colton, CA 92324 USA

来源：

CHEMICAL COMMUNICATIONS | 2024年 / 61卷 / 01期

关键词：

SELECTIVE PHOTOOXIDATION; PORPHYRIN; AGENT;

D O I：

10.1039/d4cc03890h

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Four metalloporphyrinic metal-organic frameworks (MOFs) were successfully synthesized and exhibited enhanced activities for the photooxidation of a sulfur mustard simulant, 2-chloroethyl ethyl sulfide (CEES). Among them, a Sn-porphyrin functionalized 2D MOF, namely CSLA-21-NH2(Sn), showed a half-life of 1.5 min for CEES oxidation under blue LED, featuring as one of the fastest photocatalysts for CEES degradation.

引用

页码：77 / 80

页数：5

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