PROPYLENE SELECTIVE OXIDATION AS STUDIED BY O-18 LABELING ON WELL-DEFINED MOO3 CATALYSTS

被引：0

作者：

ABON, M ^{[1
]}

ROULLET, M ^{[1
]}

MASSARDIER, J ^{[1
]}

DELICHERE, P ^{[1
]}

GUERRERORUIZ, A ^{[1
]}

机构：

[1] UNIV NACL EDUC DISTANCIA, FAC CIENCIAS, DEPT QUIM INORGAN, E-28040 MADRID, SPAIN

来源：

NEW DEVELOPMENTS IN SELECTIVE OXIDATION II | 1994年 / 82卷

关键词：

D O I：

暂无

中图分类号：

F [经济];

学科分类号：

02 ;

摘要：

The propylene oxidation reaction has been studied using O-18(2) on well defined MoO3 crystallites. Results show that the information of products -acrolein and carbon dioxide- involves the lattice oxygen. The different O-18-labelling, according to selective or total oxidation products, agrees with the structure sensitivity of this reaction. Post reaction analysis (by LRS, SIMS, LEIS) support a redox equilibrium which determines the O-18 concentration in the surface layers.

引用

页码：67 / 74

页数：8

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