Effect of Fe-loading and reaction temperature on the production of olefins from ethanol by Fe/H-ZSM-5 zeolite catalysts

被引:0
|
作者
Megumu Inaba
Kazuhisa Murata
Isao Takahara
机构
[1] National Institute of Advanced Industrial Science and Technology (AIST),
关键词
Ethanol conversion; Olefins production; Fe/H-ZSM-5 catalyst;
D O I
暂无
中图分类号
学科分类号
摘要
Lower loading of Fe (1 wt%) and higher reaction temperature (450 °C) led to higher and stable selectivity of C3+ olefins by ethanol conversion using Fe/H-ZSM-5 catalysts. Carbon deposition and framework collapse of zeolite support, which may be the cause of change in selectivity of products, was suppressed in some degree.
引用
收藏
页码:19 / 26
页数:7
相关论文
共 50 条
  • [31] Production of light olefins from methanol over modified H-ZSM-5: effect of metal impregnation in high-silica zeolite on product distribution
    Gorzin, Fatemeh
    Yaripour, Fereydoon
    RESEARCH ON CHEMICAL INTERMEDIATES, 2019, 45 (02) : 261 - 285
  • [32] Insights into the Reaction Mechanism of Ethanol Conversion into Hydrocarbons on H-ZSM-5
    Van der Borght, Kristof
    Batchu, Rakesh
    Galvita, Vladimir V.
    Alexopoulos, Konstantinos
    Reyniers, Marie-Francoise
    Thybaut, Joris W.
    Marin, Guy B.
    ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2016, 55 (41) : 12817 - 12821
  • [33] Production of light olefins from methanol over modified H-ZSM-5: effect of metal impregnation in high-silica zeolite on product distribution
    Fatemeh Gorzin
    Fereydoon Yaripour
    Research on Chemical Intermediates, 2019, 45 : 261 - 285
  • [34] Catalytic conversion of glycerol to olefins over Fe, Mo, and Nb catalysts supported on zeolite ZSM-5
    Lima, Dirleia S.
    Perez-Lopez, Oscar W.
    RENEWABLE ENERGY, 2019, 136 : 828 - 836
  • [35] Conventional hydrothermal synthesis of nanostructured H-ZSM-5 catalysts using various templates for light olefins production from methanol
    Yaripour, Fereydoon
    Shariatinia, Zahra
    Sahebdelfar, Saeed
    Irandoukht, Akbar
    JOURNAL OF NATURAL GAS SCIENCE AND ENGINEERING, 2015, 22 : 260 - 269
  • [36] Production of ethylene from hydrous ethanol on H-ZSM-5 under mild conditions
    Phillips, CB
    Datta, R
    INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 1997, 36 (11) : 4466 - 4475
  • [37] Production of ethylene from hydrous ethanol on H-ZSM-5 under mild conditions
    Univ of Iowa, Iowa City, United States
    Ind Eng Chem Res, 11 (4466-4475):
  • [38] Structure and reactivity of phosphorous modified H-ZSM-5 catalysts for ethanol dehydration
    Ramesh, Kanaparthi
    Hui, Lau Mei
    Han, Yi-Fan
    Borgna, Armando
    CATALYSIS COMMUNICATIONS, 2009, 10 (05) : 567 - 571
  • [39] DFT investigation of alkoxide formation from olefins in H-ZSM-5
    Bhan, A
    Joshi, YV
    Delgass, WN
    Thomson, KT
    JOURNAL OF PHYSICAL CHEMISTRY B, 2003, 107 (38): : 10476 - 10487
  • [40] Fe- and Cu–Zn-Containing Catalysts Based on Natural Aluminosilicate Nanotubes and Zeolite H-ZSM-5 in the Hydrogenation of Carbon Dioxide
    E. M. Smirnova
    N. D. Evdokimenko
    M. V. Reshetina
    N. R. Demikhova
    A. L. Kustov
    S. F. Dunaev
    V. A. Vinokurov
    A. P. Glotov
    Russian Journal of Physical Chemistry A, 2023, 97 : 1395 - 1401