Strong coupling between a plasmon mode and multiple different exciton states

被引:0
|
作者
Junjun Ye
Yatao Pan
Guanghui Liu
Wei Li
Renming Liu
Ming Geng
Zhixiang Liu
Zhen Chi
Xia Ran
Yanmin Kuang
Yulu He
Lijun Guo
机构
[1] Henan University,School of Physics and Electronics, Academy for Advanced Interdisciplinary Studies, International Joint Research Laboratory of New Energy Materials and Devices of Henan Province
[2] Guangdong Polytechnic Normal University,School of Optoelectronic Engineering
[3] Sun Yat-sen University,State Key Laboratory of Optoelectronic Materials and Technologies, School of Physics
来源
Science China Physics, Mechanics & Astronomy | 2023年 / 66卷
关键词
surface plasmon; strong coupling; exciton state; Rabi splitting; transient absorption; 73.20.Mf; 42.50.Pq; 73.22.-f;
D O I
暂无
中图分类号
学科分类号
摘要
Strong coupling between plasmons and multiple different exciton states (MESs) enables the creation of multiple hybrid polariton states under ambient conditions. These hybrid states possess unique optical properties different from those of their separate identities, making them ideal candidates for exploiting room-temperature multimode hybridization and multiqubit operation. In this study, we revealed the static spectral response properties of plasmon-MES strong coupling via a fully quantum mechanics approach. These theoretical predictions were experimentally demonstrated in plasmonic nanocavities containing two and three different exciton species. Additionally, the dynamical absorption processes of such strong coupling systems were investigated, and results indicated that the damping of the hybrid polariton states induced by the strong coupling could be markedly modulated by the acoustic oscillations from the plasmonic nanocavities. Our findings contribute a theoretical approach for accurately describing the plasmon-MES interactions and a platform for developing the high-speed active plasmonic devices based on multiqubit strong coupling.
引用
收藏
相关论文
共 50 条
  • [31] Surface Plasmon Mediated Strong Exciton-Photon Coupling in Semiconductor Nanocrystals
    Gomez, D. E.
    Vernon, K. C.
    Mulvaney, P.
    Davis, T. J.
    NANO LETTERS, 2010, 10 (01) : 274 - 278
  • [32] Nanoscale quantum plasmon sensing based on strong photon-exciton coupling
    Qian, Zhiyuan
    Ren, Juanjuan
    Zhang, Fan
    Duan, Xueke
    Gong, Qihuang
    Gu, Ying
    NANOTECHNOLOGY, 2020, 31 (12)
  • [33] Strong coupling in molecular exciton-plasmon Au nanorod array systems
    Fedele, Stefano
    Hakami, Manal
    Murphy, Antony
    Pollard, Robert
    Rice, James
    APPLIED PHYSICS LETTERS, 2016, 108 (05)
  • [34] Strong Exciton-Plasmon Coupling in Waveguide-Based Plexcitonic Nanostructures
    Mahinroosta, Tayebeh
    Mehri Hamidi, Seyedeh
    PHYSICA STATUS SOLIDI B-BASIC SOLID STATE PHYSICS, 2020, 257 (12):
  • [35] Exciton-Plasmon Energy Exchange Drives the Transition to a Strong Coupling Regime
    Shahbazyan, Tigran V.
    NANO LETTERS, 2019, 19 (05) : 3273 - 3279
  • [36] Particularities of surface plasmon-exciton strong coupling with large Rabi splitting
    Symonds, C.
    Bonnand, C.
    Plenet, J. C.
    Brehier, A.
    Parashkov, R.
    Lauret, J. S.
    Deleporte, E.
    Bellessa, J.
    NEW JOURNAL OF PHYSICS, 2008, 10
  • [37] Molecular plasmonics: The role of rovibrational molecular states in exciton-plasmon materials under strong-coupling conditions
    Sukharev, Maxim
    Charron, Eric
    PHYSICAL REVIEW B, 2017, 95 (11)
  • [38] Tunable strong plasmon-exciton coupling between single silver nanocube dimer and J-aggregates
    Li, Chao
    Wu, Fan
    Jiang, Ping
    Wang, Yilin
    Wang, Lulu
    Yu, Li
    PHYSICA B-CONDENSED MATTER, 2019, 569 : 40 - 47
  • [39] Strong Coupling between Surface Plasmon Resonance and Exciton of Labeled Protein-Dye Complex for Immunosensing Applications
    Jurksaitis, Povilas
    Buzavaite-Verteliene, Ernesta
    Balevicius, Zigmas
    INTERNATIONAL JOURNAL OF MOLECULAR SCIENCES, 2023, 24 (03)
  • [40] Plasmon/exciton and plasmon/photonic mode interaction
    Schatz, George
    ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY, 2015, 249