The longevity of cratons is generally attributed to persistence of
neutrally-to-positively buoyant and mechanically strong lithosphere that shields the
cratonic crust from underlying mantle dynamics. Here we show that large portions of
the cratonic lithosphere in South America and Africa, however, experienced
significant modification during and since the Mesozoic era, as demonstrated by
widespread Cretaceous uplift and volcanism, present-day high topography, thin crust,
and the presence of seismically fast but neutrally buoyant upper-mantle anomalies.
We suggest that these observations reflect a permanent increase in lithospheric
buoyancy due to plume-triggered delamination of deep lithospheric roots during the
Late Cretaceous and early Cenozoic periods. Lithosphere in these regions has been
thermally reestablished since then, as confirmed by its present-day low heat flow,
high seismic velocities and realigned seismic anisotropy. We conclude that the
original lowermost cratonic lithosphere is compositionally denser than the
asthenospheric mantle and can be removed when perturbed by underlying mantle
upwelling. Therefore, it is the buoyancy of the upper lithosphere that perpetuates
stabilization of cratons.