A mathematical model to describe the alpha dose rate from a UO2 surface

被引:5
|
作者
Siberry, Angus [1 ]
Hambley, David [2 ]
Adamska, Anna [3 ]
Springell, Ross [1 ]
机构
[1] Univ Bristol, HH Wills Phys Lab, Bristol BS8 1TL, Avon, England
[2] Natl Nucl Lab Ltd, Cent Lab, Sellafield CA20 1PG, Cumbria, England
[3] Sellafield Ltd, Sir Christopher Harding House, Whitehaven CA28 7XY, England
基金
英国工程与自然科学研究理事会;
关键词
Alpha radiation; Dosimetry; UO2; Radiolysis; SRIM; Spent Fuel; SPENT NUCLEAR-FUEL; STOPPING POWER; RATE PROFILE; WATER; DISSOLUTION; RADIOLYSIS; CONTACT; CORROSION; PROTONS; ENERGY;
D O I
10.1016/j.radphyschem.2021.109359
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
A model to determine the dose rate of a planar alpha-emitting surface has been developed. The approach presented is a computationally efficient mathematical model using stopping range data from the Stopping Ranges of Ions in Matter (SRIM) software. The alpha dose rates as a function of distance from irradiated UO2 spent fuel surfaces were produced for benchmarking with previous modelling attempts. This method is able to replicate a Monte Carlo (MCNPX) study of an irradiated UO2 fuel surface within 0.6% of the resulting total dose rate and displays a similar dose profile.
引用
收藏
页数:8
相关论文
共 50 条
  • [31] Electrolytic reduction rate of porous UO2 pellets
    Jeon, Min Ku
    Choi, Eun-Young
    Kim, Sung-Wook
    Lee, Sang-Kwon
    Kang, Hyun Woo
    Hong, Sun Seok
    Lee, Jeong
    Hur, Jin-Mok
    Jeon, Sang-Chae
    Lee, Ju Ho
    Cho, Yung-Zun
    Ahn, Do-Hee
    KOREAN JOURNAL OF CHEMICAL ENGINEERING, 2016, 33 (07) : 2235 - 2239
  • [32] Electrolytic reduction rate of porous UO2 pellets
    Min Ku Jeon
    Eun-Young Choi
    Sung-Wook Kim
    Sang-Kwon Lee
    Hyun Woo Kang
    Sun Seok Hong
    Jeong Lee
    Jin-Mok Hur
    Sang-Chae Jeon
    Ju Ho Lee
    Yung-Zun Cho
    Do-Hee Ahn
    Korean Journal of Chemical Engineering, 2016, 33 : 2235 - 2239
  • [33] DISSOLUTION RATE-EQUATION OF UO2 PELLET
    HOMMA, S
    KOGA, J
    MATSUMOTO, S
    KAWATA, T
    JOURNAL OF NUCLEAR SCIENCE AND TECHNOLOGY, 1993, 30 (09) : 959 - 961
  • [34] INFLUENCE OF STOICHIOMETRY ON THE RATE OF GRAIN GROWTH OF UO2
    AMATO, I
    COLOMBO, RL
    PROTTI, AM
    JOURNAL OF THE AMERICAN CERAMIC SOCIETY, 1963, 46 (08) : 407 - 407
  • [35] Effect of surface orientation on dissolution rate and surface dynamics of UO2 single crystals in nitric acid
    Bertolotto, Solene
    Szenknect, Stephanie
    Lalleman, Sophie
    Magnaldo, Alastair
    Raison, Philippe
    Odorico, Michael
    Podor, Renaud
    Claparede, Laurent
    Dacheux, Nicolas
    CORROSION SCIENCE, 2020, 176
  • [36] Influence of alpha radiolysis of water on UO2 matrix alteration:: Chemical/transport model
    Poulesquen, A.
    Jegou, C.
    NUCLEAR TECHNOLOGY, 2007, 160 (03) : 337 - 345
  • [37] A continuum model for cracked UO2 fuel
    Jernkvist, LO
    NUCLEAR ENGINEERING AND DESIGN, 1997, 176 (03) : 273 - 284
  • [38] MODEL FOR IN-REACTOR DENSIFICATION OF UO2
    MACEWEN, SR
    HASTINGS, IJ
    PHILOSOPHICAL MAGAZINE, 1975, 31 (01) : 135 - 143
  • [39] A STATISTICAL THERMODYNAMIC MODEL FOR NONSTOICHIOMETRIC UO2
    AITKEN, EA
    FRYXELL, RE
    AMERICAN CERAMIC SOCIETY BULLETIN, 1965, 44 (04): : 391 - &
  • [40] Conceptual and mathematical model for the UO2(s) dissolution in brines under different redox conditions
    Gimenez, J
    de Pablo, J
    Torrero, ME
    Casas, I
    RADIOCHIMICA ACTA, 1997, 78 : 21 - 25