Inorganic chemical composition and source signature of PM2.5 in Beijing during ACE-Asia period

被引:39
|
作者
Zhang, RJ [1 ]
Xu, YF [1 ]
Han, ZW [1 ]
机构
[1] Chinese Acad Sci, Inst Atmospher Phys, LAPC, Beijing 100029, Peoples R China
来源
CHINESE SCIENCE BULLETIN | 2003年 / 48卷 / 10期
关键词
dust; ACE-Asia; PM2.5; chemical composition; source apportionment;
D O I
10.1360/02wd0375
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
Aerosol samples for PM2.5 were collected in Beijing for 38 consecutive days from March to April 2001 using an IMPROVE Sampler. Concentrations of 20 elements in PM2.5 were determined using a PIXE method. Results show that the average mineral dust concentration Of PM2.5 was 14.6 mug/m(3) during the observation period. On the sand-dust event days of March 21 and April 10, dust PM2.5 mass concentrations were 62.4 and 54.1 mug/m(3), respectively. These demonstrate that fine particle pollution by dust event in Beijing was very severe. The enrichment factors of S and Cu reached minimums on the dusty days and were high on the non-dusty days. It is considered that enrichment factors of elements in PM2.5, which are associated with human activities, can probably provide an effective method to distinguish local sources from external sources of dust. Factor analysis on the chemical composition in PM2.5 shows that sources of crustal matters, anthropogenic emission, and oil combustion contributed to PM2.5 levels in air in the springtime of 2001 in Beijing.
引用
收藏
页码:1002 / 1005
页数:4
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