Tuning the optical properties of the zirconium-UiO-66 metal-organic framework for photocatalytic degradation of methyl orange

被引：92
|
作者：
Pu, Shan [1 ]
Xu, Lei [1 ]
Sun, Lin [1 ]
Du, Hongbin [1 ]
机构：
[1] Nanjing Univ, Sch Chem & Chem Engn, State Key Lab Coordinat Chem, Nanjing 210093, Jiangsu, Peoples R China
来源：
INORGANIC CHEMISTRY COMMUNICATIONS | 2015年 / 52卷
基金：
中国国家自然科学基金;
关键词：
MOFs; Zirconium; UiO-66; analogs; Photocatalysis; Degradation of methyl orange; CO2; REDUCTION; BLUE DYE; DECOLORIZATION;
D O I：
10.1016/j.inoche.2014.12.015
中图分类号：
O61 [无机化学];
学科分类号：
070301 ; 081704 ;
摘要：
A new UiO-66-type zirconium metal organic framework material UiO-66(AN) was prepared by using chromophoric anthracene-9,10-dicarboxylic acid as linker. The large-sized conjugate pi-system in the ligand results in the bathochromic shift of the absorption peaks into the visible light region in the absorption spectrum of UiO-66(AN), compared to those of UiO-66 and analogs UiO-66(NA) made of terephthalate and naphthalene-1,4-dicarboxylic add, respectively. UiO-66(AN) was shown to be an efficient photocatalyst for degradation of methyl orange. Our finding shows promises for the development of more efficient MOFs as photocatalysts by using chromophoric conjugate ligands. (C) 2014 Elsevier B.V. All rights reserved.
引用
收藏
页码：50 / 52
页数：3
相关论文
共 50 条
  • [31] Improving photocatalytic hydrogen production of metal-organic framework UiO-66 octahedrons by dye-sensitization
    Yuan, Yu-Peng
    Yin, Li-Sha
    Cao, Shao-Wen
    Xu, Geng-Sheng
    Li, Chuan-Hao
    Xue, Can
    APPLIED CATALYSIS B-ENVIRONMENTAL, 2015, 168 : 572 - 576
  • [32] Diastereoselective Synthesis of Pyranoquinolines on Zirconium Containing UiO-66 Metal-Organic Frameworks
    Rechac, Victor L.
    Cirujano, Francisco G.
    Corma, Avelino
    Llabres i Xamena, Francesc X.
    EUROPEAN JOURNAL OF INORGANIC CHEMISTRY, 2016, (27) : 4512 - 4516
  • [33] Strain Engineering for Tuning the Photocatalytic Activity of Metal-Organic Frameworks-Theoretical Study of the UiO-66 Case
    Stojkovic, Marija
    Pasti, Igor A.
    CATALYSTS, 2021, 11 (02) : 1 - 10
  • [34] Computational study of Bronsted acidity in the metal-organic framework UiO-66
    Chen, Haoyuan
    CHEMICAL PHYSICS LETTERS, 2022, 800
  • [35] Exceptional Mechanical Stability of Highly Porous Zirconium Metal-Organic Framework UiO-66 and Its Important Implications
    Wu, Hui
    Yildirim, Taner
    Zhou, Wei
    JOURNAL OF PHYSICAL CHEMISTRY LETTERS, 2013, 4 (06): : 925 - 930
  • [36] Synthesis and hydrogen storage studies of metal-organic framework UiO-66
    Zhao, Qiang
    Yuan, Wen
    Liang, Jianming
    Li, Jinping
    INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2013, 38 (29) : 13104 - 13109
  • [37] Memristive behavior of UiO-66 metal-organic framework single crystal
    Bachinin, Semyon V.
    Lubimova, Anastasia
    Povarov, Svyatoslav A.
    Zubok, Dmitrii
    Okoneshnikova, Elizaveta
    Kulakova, Alena N.
    Rzhevskiy, Sergey S.
    Milichko, Valentin A.
    PHOTONICS AND NANOSTRUCTURES-FUNDAMENTALS AND APPLICATIONS, 2024, 58
  • [38] On the intrinsic dynamic nature of the rigid UiO-66 metal-organic framework
    Hajek, Julianna
    Caratelli, Chiara
    Demuynck, Ruben
    De Wispelaere, Kristof
    Vanduyfhuys, Louis
    Waroquier, Michel
    Van Speybroeck, Veronique
    CHEMICAL SCIENCE, 2018, 9 (10) : 2723 - 2732
  • [39] Chlorine retention in drinking water with UiO66 metal-organic framework
    Serrano-Palafox, Sergio A.
    Romero-Romero, Fernando
    Varela-Guerrero, Victor
    Ballesteros-Rivas, Maria F.
    BULLETIN OF MATERIALS SCIENCE, 2024, 47 (01)
  • [40] Free Energy of Ligand Removal in the Metal-Organic Framework UiO-66
    Bristow, Jessica K.
    Svane, Katrine L.
    Tiana, Davide
    Skelton, Jonathan M.
    Gale, Julian D.
    Walsh, Aron
    JOURNAL OF PHYSICAL CHEMISTRY C, 2016, 120 (17): : 9276 - 9281
12345