Pt/C trapped in activated graphitic carbon layers as a highly durable electrocatalyst for the oxygen reduction reaction

被引:80
|
作者
Nie, Yao [1 ]
Chen, Siguo [1 ]
Ding, Wei [1 ]
Xie, Xiaohong [1 ]
Zhang, Yun [1 ]
Wei, Zidong [1 ]
机构
[1] Chongqing Univ, Coll Chem & Chem Engn, State Key Lab Power Transmiss Equipment & Syst Se, Chongqing 400044, Peoples R China
关键词
MEMBRANE FUEL-CELLS; CATALYTIC-ACTIVITY; NANOPARTICLES; POLYANILINE; CORROSION; ALLOY; IRON; ELECTROLYTE; OPERATION; SURFACES;
D O I
10.1039/c4cc06781a
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
A thin nitrogen-doped graphitic carbon layer is elaborately introduced into the Pt/C surface to not only inhibit migration and dissolution of Pt nanoparticles, but also impart activity to the integral catalyst without blocking the inner Pt catalytic active sites. The corrosion of the carbon support can also be alleviated due to the outer graphitic coverage.
引用
收藏
页码:15431 / 15434
页数:4
相关论文
共 50 条
  • [41] A chromium nitride/carbon nitride containing graphitic carbon nanocapsule hybrid as a Pt-free electrocatalyst for oxygen reduction
    Zhao, Lu
    Wang, Lei
    Yu, Peng
    Zhao, Dongdong
    Tian, Chungui
    Feng, He
    Ma, Jing
    Fu, Honggang
    CHEMICAL COMMUNICATIONS, 2015, 51 (62) : 12399 - 12402
  • [42] Nitrogen doped lotus stem carbon as electrocatalyst comparable to Pt/C for oxygen reduction reaction in alkaline media
    Weththasinha, H. A. B. M. D.
    Yan, Zaoxue
    Gao, Lina
    Li, Yuan
    Pan, Denghui
    Zhang, Mingmei
    Lv, Xiaomeng
    Wei, Wei
    Xie, Jimin
    INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2017, 42 (32) : 20560 - 20567
  • [43] Effect of carbon nanofiber surface groups on oxygen reduction reaction of supported Pt electrocatalyst
    Zhong, Ren-Sheng
    Qin, Yuan-Hang
    Niu, Dong-Fang
    Zhang, Xin-Sheng
    Zhou, Xin-Gui
    Sun, Shi-Gang
    Yuan, Wei-Kang
    ELECTROCHIMICA ACTA, 2013, 89 : 157 - 162
  • [44] Mechanistic study on nitrogen-doped graphitic carbon-reinforced chromium nitride as a durable electrocatalyst for oxygen reduction
    Sarkar, Bidushi
    Parui, Arko
    Singh, Abhishek Kumar
    Nanda, Karuna Kar
    JOURNAL OF MATERIALS CHEMISTRY A, 2021, 9 (30) : 16575 - 16584
  • [45] One-step Synthesis of Pt Nanoparticles Highly Loaded on Graphene Aerogel as Durable Oxygen Reduction Electrocatalyst
    Huang, Qinghong
    Tao, Feifei
    Zou, Liangliang
    Yuan, Ting
    Zou, Zhiqing
    Zhang, Haifeng
    Zhang, Xiaogang
    Yang, Hui
    ELECTROCHIMICA ACTA, 2015, 152 : 140 - 145
  • [46] Direct synthesis of a carbon nanotube interpenetrated doped porous carbon alloy as a durable Pt-free electrocatalyst for the oxygen reduction reaction in an alkaline medium
    Unni, Sreekuttan M.
    Anilkumar, Gopinathan M.
    Matsumoto, Masashi
    Tamaki, Takanori
    Imai, Hideto
    Yamaguchi, Takeo
    SUSTAINABLE ENERGY & FUELS, 2017, 1 (07): : 1524 - 1532
  • [47] A highly active and durable iron/cobalt alloy catalyst encapsulated in N-doped graphitic carbon nanotubes for oxygen reduction reaction
    An, Li
    Jiang, Ning
    Li, Biao
    Hua, Shixin
    Fu, Yutong
    Liu, Jiaxi
    Hao, Wei
    Xia, Dingguo
    Sun, Zaicheng
    JOURNAL OF MATERIALS CHEMISTRY A, 2018, 6 (14) : 5962 - 5970
  • [48] CoFe alloy embedded in N-doped carbon nanotubes derived from triamterene as a highly efficient and durable electrocatalyst beyond commercial Pt/C for oxygen reduction
    Meng, Hong-Ling
    Lin, Shi-Yi
    Cao, Ying
    Wang, Ai-Jun
    Zhang, Lu
    Feng, Jiu-Ju
    JOURNAL OF COLLOID AND INTERFACE SCIENCE, 2021, 604 : 856 - 865
  • [49] Facile Route to Synthesize Cu, S, N-Doped Carbon as Highly Efficient and Durable Electrocatalyst Towards Oxygen Reduction Reaction
    Zhao, Yiwei
    Yu, Yue
    Wang, Yuanhong
    Ma, Jicheng
    Xing, Shuangxi
    CATALYSIS LETTERS, 2022, 152 (08) : 2342 - 2351
  • [50] Facile Route to Synthesize Cu, S, N-Doped Carbon as Highly Efficient and Durable Electrocatalyst Towards Oxygen Reduction Reaction
    Yiwei Zhao
    Yue Yu
    Yuanhong Wang
    Jicheng Ma
    Shuangxi Xing
    Catalysis Letters, 2022, 152 : 2342 - 2351