Theoretical and experimental approaches to enhanced two-photon absorption

被引：0
|
作者：
Kamada, Kenji [1 ]
Ohta, Koji [1 ]
机构：
[1] Natl Inst Ind Sci & Technol AIST, Photon Res Inst, AIST Kansai Ctr, 1-8-31 Midorigaoka, Ikeda, Osaka 8638577, Japan
来源：
ORGANIC PHOTONIC MATERIALS AND DEVICES IX | 2007年 / 6470卷
关键词：
two-photon absorption; resonance enhancement; alternancy symmetry; structure-property relationship;
D O I：
10.1117/12.707830
中图分类号：
T [工业技术];
学科分类号：
08 ;
摘要：
A selection rule for two-photon transition is considered based on the alternancy symmetry and the result is adopted to explain the experimental and calculation results of two-photon absorption (TPA) properties of two diacetylene derivatives with neutral and charged peripheral groups. The discussion successfully explains the difference in strength of the TPA bands and the existence of the higher-lying TPA states that is strongly allowed and plays a main role to the resonance enhancement of TPA.
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页数：8
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