Surface dynamics of polymer films -: art. no. 068302

被引:170
|
作者
Kim, H [1 ]
Rühm, A
Lurio, LB
Basu, JK
Lal, J
Lumma, D
Mochrie, SGJ
Sinha, SK
机构
[1] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA
[2] Univ Calif San Diego, Dept Phys, La Jolla, CA 92093 USA
[3] Los Alamos Natl Lab, LANSCE, Los Alamos, NM 87545 USA
[4] Sogang Univ, Dept Phys, Seoul 121742, South Korea
[5] MIT, Ctr Mat Sci & Engn, Cambridge, MA 02139 USA
[6] Max Planck Inst Met Res, Stuttgart, Germany
[7] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA
[8] Univ Illinois, Mat Res Lab, Urbana, IL 61801 USA
[9] Argonne Natl Lab, Intense Pulsed Neutron Source, Argonne, IL 60439 USA
[10] Yale Univ, Dept Phys & Appl Phys, New Haven, CT 06520 USA
关键词
D O I
10.1103/PhysRevLett.90.068302
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
The dynamics of supported polymer films were studied by probing the surface height fluctuations as a function of lateral length scale using x-ray photon correlation spectroscopy. Measurements were performed on polystyrene (PS) films of thicknesses varying from 84 to 333 nm at temperatures above the PS glass transition temperature. Within a range of wave vectors spanning 10(-3) to 10(-2) nm(-1), good agreement is found between the measured surface dynamics and the theory of overdamped thermal capillary waves on thin films. Quantitatively, the data can be accounted for using the viscosity of bulk PS.
引用
收藏
页数:4
相关论文
共 50 条
  • [41] Resonant photoemission of TiN films -: art. no. 075403
    Fuentes, GG
    Prieto, P
    Morant, C
    Quirós, C
    Núñez, R
    Soriano, L
    Elizalde, E
    Sanz, JM
    PHYSICAL REVIEW B, 2001, 63 (07):
  • [42] Stochastic gain in population dynamics -: art. no. 028701
    Traulsen, A
    Röhl, T
    Schuster, HG
    PHYSICAL REVIEW LETTERS, 2004, 93 (02) : 028701 - 1
  • [43] Matter and dynamics in closed cosmologies -: art. no. 083506
    Heinzle, JM
    Röhr, N
    Uggla, C
    PHYSICAL REVIEW D, 2005, 71 (08): : 1 - 17
  • [44] Ab initio Ehrenfest dynamics -: art. no. 084106
    Li, XS
    Tully, JC
    Schlegel, HB
    Frisch, MJ
    JOURNAL OF CHEMICAL PHYSICS, 2005, 123 (08):
  • [45] Optimal estimation of quantum dynamics -: art. no. 050302
    Acín, A
    Jané, E
    Vidal, G
    PHYSICAL REVIEW A, 2001, 64 (05): : 4
  • [46] Influence of trapping on the exciton dynamics of AlxGa1-xAs films -: art. no. 111906
    Amo, A
    Martin, MD
    Klopotowski, L
    Viña, L
    Toropov, AI
    Zhuravlev, KS
    APPLIED PHYSICS LETTERS, 2005, 86 (11) : 1 - 3
  • [47] Nonadiabatic simulations of polaron dynamics -: art. no. 235205
    Johansson, AA
    Stafström, S
    PHYSICAL REVIEW B, 2004, 69 (23) : 235205 - 1
  • [48] Smoothed dissipative particle dynamics -: art. no. 026705
    Español, P
    Revenga, M
    PHYSICAL REVIEW E, 2003, 67 (02):
  • [49] Molecular dynamics in polymeric systems -: art. no. 044
    Dionísio, M
    Alves, NM
    Mano, JF
    E-POLYMERS, 2004,
  • [50] Relaxation dynamics of magic clusters -: art. no. 035421
    Kim, YD
    Niemietz, M
    Gerhardt, P
    von Gynz-Rekowski, F
    Ganteför, G
    PHYSICAL REVIEW B, 2004, 70 (03): : 035421 - 1