Lattice-Boltzmann simulation of coalescence-driven island coarsening

被引:6
|
作者
Basagaoglu, H [1 ]
Green, CT
Meakin, P
McCoy, BJ
机构
[1] Idaho Natl Lab, Idaho Falls, ID 83415 USA
[2] US Geol Survey, Menlo Pk, CA 94025 USA
[3] Louisiana State Univ, Dept Chem Engn, Baton Rouge, LA 70803 USA
来源
JOURNAL OF CHEMICAL PHYSICS | 2004年 / 121卷 / 16期
关键词
D O I
10.1063/1.1804158
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
A two-dimensional lattice-Boltzmann model (LBM) with fluid-fluid interactions was used to simulate first-order phase separation in a thin fluid film. The intermediate asymptotic time dependence of the mean island size, island number concentration, and polydispersity were determined and compared with the predictions of the distribution-kinetics model. The comparison revealed that the combined effects of growth, coalescence, and Ostwald ripening control the phase transition process in the LBM simulations. However, the overall process is dominated by coalescence, which is independent of island mass. As the phase transition advances, the mean island size increases, the number of islands decrease, and the polydispersity approaches unity, which conforms to the predictions of the distribution-kinetics model. The effects of the domain size on the intermediate asymptotic island size distribution, scaling form of the island size distribution, and the crossover to the long-term asymptotic behavior were elucidated. (C) 2004 American Institute of Physics.
引用
收藏
页码:7987 / 7995
页数:9
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