An explanation of the density maximum in water

被引：105

作者：

Cho, CH ^{[1
]}

Singh, S ^{[1
]}

Robinson, GW ^{[1
]}

机构：

[1] TEXAS TECH UNIV, DEPT PHYS, LUBBOCK, TX 79409 USA

来源：

PHYSICAL REVIEW LETTERS | 1996年 / 76卷 / 10期

关键词：

D O I：

10.1103/PhysRevLett.76.1651

中图分类号：

O4 [物理学];

学科分类号：

0702 ;

摘要：

An explanation of the anomalous density maximum in water near 4 degrees C can be given in terms of a competition between the presence of open second-neighbor oxygen-oxygen structure at 4.5 Angstrom and a dense second-neighbor structure obtained from the bending of hydrogen bonds. Since no computational model of water has provided an explanation of this anomaly, altering the water-water potential to create more realistic interactions in the second-neighbor shell is proposed. Support for this idea is provided here by considering the exactly soluble Takahashi fluid model.

引用

页码：1651 / 1654

页数：4

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