One-step synthesis of cobalt, nitrogen-codoped carbon as nonprecious bifunctional electrocatalyst for oxygen reduction and evolution reactions

被引：54

作者：

Guo, Sijie ^{[1
]}

Yang, Yanmei ^{[1
]}

Liu, Naiyun ^{[1
]}

Qiao, Shi ^{[1
]}

Huang, Hui ^{[1
]}

Liu, Yang ^{[1
]}

Kang, Zhenhui ^{[1
]}

机构：

[1] Soochow Univ, Inst Funct Nano & Soft Mat FUNSOM, Jiangsu Key Lab Carbon Based Funct Mat & Devices, Suzhou 215123, Peoples R China

来源：

SCIENCE BULLETIN | 2016年 / 61卷 / 01期

基金：

中国国家自然科学基金;

关键词：

Carbon quantum dots; Bifunctional catalyst; Electrochemical performance; MEMBRANE FUEL-CELL; DOPED GRAPHENE; QUANTUM DOTS; FACILE SYNTHESIS; WATER OXIDATION; VISIBLE-LIGHT; CATALYST; COMPOSITE; NANOPARTICLES; PERFORMANCE;

D O I：

10.1007/s11434-015-0978-6

中图分类号：

O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];

学科分类号：

07 ; 0710 ; 09 ;

摘要：

It is highly desired for the development of efficient bifunctional electrocatalyst for both oxygen reduction reaction (ORR) and oxygen evolution reaction (OER) in renewable energy technologies. In this work, cobalt, nitrogen-codoped carbon was prepared by a facile one-step method and demonstrated to exhibit good electrocatalytic performance for ORR and OER via a complete four-electron process. Besides, the catalyst prepared at 900 degrees C also displayed excellent stability for both ORR and OER. Furthermore, the origin of catalytic activity was also explored, which was attributed to the synergistic effects of metallic Co and quaternary N.

引用

页码：68 / 77

页数：10

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