Efficient separation of vitamins mixture in aqueous solution using a stable zirconium-based metal-organic framework

被引：22
|
作者：
Zhao, Xudong [1 ]
Zhao, Yuwei [1 ]
Zheng, Meiqi [1 ]
Liu, Shuangxue [1 ]
Xue, Wenjuan [2 ]
Du, Guohua [1 ]
Wang, Ting [1 ]
Gao, Xinli [3 ]
Wang, Keke [4 ]
Hu, Jianshui [1 ]
Gao, Zhuqing [1 ]
Huang, Hongliang [2 ]
机构：
[1] Taiyuan Univ Sci & Technol, Coll Chem & Biol Engn, Taiyuan 030024, Shanxi, Peoples R China
[2] Tianjin Polytech Univ, Natl Ctr Int Joint Res Separat Membranes, State Key Lab Separat Membranes & Membrane Proc, Tianjin 300387, Peoples R China
[3] Taiyuan Univ Sci & Technol, Instrumental Anal Ctr, Taiyuan 030024, Shanxi, Peoples R China
[4] Zhejiang Univ Technol, Coll Chem Engn, State Key Lab Breeding Base Green Chem Synth Tech, Hangzhou 310014, Zhejiang, Peoples R China
来源：
JOURNAL OF COLLOID AND INTERFACE SCIENCE | 2019年 / 555卷
基金：
中国国家自然科学基金;
关键词：
Metal-organic framework; Separation; B-vitamins; Electrostatic interaction; BASIS-SETS; NICOTINIC-ACID; REMOVAL; PERFORMANCE; ADSORPTION; OXIDATION; NIACIN; MOFS;
D O I：
10.1016/j.jcis.2019.08.024
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
High-efficiency separation of niacin (NIA) and nicotinamide (NIC) still faces large challenge up to date. In this work, a stable zirconium-based metal-organic framework (DUT-67) was used to adsorb and separate NIA and NIC in aqueous solutions. The adsorption capacities for NIA and NIC at the concentration ratio of 1:1 were 110.2 mg g(-1) and 11.2 mg g(-1) respectively. Further study indicates that low ratio of NIA/NIC is in favor of the separation. High temperature can restrain the adsorptions of NIA and NIC but promote the separation. Besides, DUT-67 can be well regenerated via a simple method. Mechanism analysis indicates that electrostatic interaction plays a critical role in the separation of these vitamins. (C) 2019 Elsevier Inc. All rights reserved.
引用
收藏
页码：714 / 721
页数：8
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