3D porous Ti3C2Tx MXene/rGO/SnO2 aerogel for formaldehyde detection at room temperature

被引:20
|
作者
Liu, Miao [1 ]
Song, Peng [1 ]
Liang, Dong [1 ]
Ding, Yongling [2 ]
Wang, Qi [1 ]
机构
[1] Univ Jinan, Sch Mat Sci & Engn, Jinan 250022, Peoples R China
[2] Shandong Jiaotong Univ, Sch Transportat Civil Engn, Jinan 250357, Peoples R China
基金
中国国家自然科学基金;
关键词
Ti(3)C(2)Tx MXene aerogel; SnO2; Reduced graphene oxide; Formaldehyde; Gas sensor; Room temperature; GAS SENSOR; NANOCOMPOSITES;
D O I
10.1016/j.jallcom.2022.166664
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The high-performance formaldehyde sensor is an ideal choice for industrial gas detection and environmental gas analysis. In this article, the 3D Ti3C2Tx MXene/rGO/SnO2 aerogle was successfully fabricated via a simple one-step solvothermal route. The composite structures and morphology were characterized by an array of testing techniques. According to the gas measurement, the 3D Ti3C2Tx MXene/rGO/SnO2 sensor exhibited 54.97% sensing response in 10 ppm formaldehyde at room temperature (RT). Not only that, the 3D Ti3C2Tx MXene/rGO/SnO2-based sensor indicated an excellent sensing selectivity, short response and recovery times (2.9 and 2.2 s, separately), good repeatability and stability. A general formaldehyde sensing mechanism with a ternary architectural was proposed and supported through density functional theory (DFT) calculations data, which has been sufficiently shown to be a promising candidate for the design of efficient formaldehyde sensor. (c) 2022 Elsevier B.V. All rights reserved.
引用
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页数:10
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