Mixing in reaction dynamics under enhanced diffusion conditions

被引:5
|
作者
Zumofen, G
Klafter, J
Shlesinger, MF
机构
[1] TEL AVIV UNIV, SCH CHEM, IL-69978 TEL AVIV, ISRAEL
[2] OFF NAVAL RES, DIV PHYS, ARLINGTON, VA 22217 USA
来源
关键词
D O I
10.1016/S0370-1573(97)00065-3
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We first review the Levy-flight approach for the description of enhanced diffusion and then study the effects of mixing on the transient A + B --> 0 reaction at stoichiometric conditions in d = 1-3 dimensions under enhanced diffusion conditions; The particles are assumed to follow Levy walks, characterized by an index , which result in enhanced diffusion for 1 < gamma < 2. Particle density decays and particle-particle correlation functions are calculated using deterministic reaction-diffusion equations and computer simulations of this multi-particle problem. We concentrate on the segregation phenomenon and demonstrate that, depending on gamma, segregation may disappear in d = 3 dimensions under enhanced diffusion conditions. Hence, Levy walks lead to an efficient mixing of reacting particles.
引用
收藏
页码:157 / 171
页数:15
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