Ternary photocatalyst of atomic-scale Pt coupled with MoS2 co-loaded on TiO2 surface for highly efficient degradation of gaseous toluene

被引:58
|
作者
Qu, Jiafu [1 ]
Chen, Dongyun [1 ]
Li, Najun [1 ]
Xu, Qingfeng [1 ]
Li, Hua [1 ]
He, Jinghui [1 ]
Lu, Jianmei [1 ]
机构
[1] Soochow Univ, Collaborat Innovat Ctr Suzhou Nano Sci & Technol, Coll Chem Chem Engn & Mat Sci, Suzhou 215123, Peoples R China
基金
国家重点研发计划; 中国国家自然科学基金;
关键词
TiO2; nanosheets; Molybdenum disulfide; Atomic-scale Pt; Photocatalytic oxidation; Toluene removal; SINGLE-ATOM; OXIDATION; NANOSHEETS; PHOTODEGRADATION; HETEROJUNCTIONS; NANOCOMPOSITES; NANOPARTICLES; IRRADIATION; ADSORPTION; COCATALYST;
D O I
10.1016/j.apcatb.2019.117877
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Photocatalysis by semiconducting materials loaded with non-metal or noble metals is an excellent strategy for removal of gaseous toluene. Herein, a new photocatalytic system was successfully prepared via simultaneously coupling atomic-scale Pt with MoS2 as co-catalysts to load on the surface of TiO2. The obtained photocatalysts exhibited good performance in toluene degradation by promoting the separation of photogenerated electron-hole pairs. The most efficient toluene degradation was achieved by the photocatalyst with a content of 2.0 wt% Pt-MT-1.0 (i.e., coupling 2.0 wt% atomic-scale Pt with 1.0 wt% MoS2), with a conversion ratio of 91.5%. This conversion ratio was higher than those of platinum-free MT-1.0 (33.9%) and pure TiO2 (72.3%). The results demonstrate the potential application of this new nanocomposite for efficient photocatalytic degradation of toluene.
引用
收藏
页数:8
相关论文
共 50 条
  • [11] TiO2 coupled to predominantly metallic MoS2 for photocatalytic degradation of rhodamine B
    Yangyang Wang
    Shengrui Sun
    Yangqiao Liu
    Yuzhi Zhang
    Jinfeng Xia
    Qingfeng Yang
    Journal of Materials Science, 2020, 55 : 12274 - 12286
  • [12] Isolated Pt single atomic sites anchored on nanoporous TiO2 film for highly efficient photocatalytic degradation of low concentration toluene
    Xu, Tongzhou
    Zheng, Hong
    Zhang, Pengyi
    JOURNAL OF HAZARDOUS MATERIALS, 2020, 388 (388)
  • [13] TiO2 nanorod decorated with MoS2 nanospheres: An efficient dual-functional photocatalyst for antibiotic degradation and hydrogen production
    Govinda raj M.
    Mahalingam S.
    Gnanarani S.V.
    Jayashree C.
    Ganeshraja A.S.
    Pugazhenthiran N.
    Rahaman M.
    Abinaya S.
    Senthil B.
    Kim J.
    Chemosphere, 2024, 357
  • [14] Synthesis of Immobilized CdS/TiO2 Nanofiber Heterostructure Photocatalyst for Efficient Degradation of Toluene
    Mengmeng Zhang
    Meng Liu
    Yan Jiang
    Jingying Li
    Qinghua Chen
    Water, Air, & Soil Pollution, 2020, 231
  • [15] Synthesis of Immobilized CdS/TiO2 Nanofiber Heterostructure Photocatalyst for Efficient Degradation of Toluene
    Zhang, Mengmeng
    Liu, Meng
    Jiang, Yan
    Li, Jingying
    Chen, Qinghua
    WATER AIR AND SOIL POLLUTION, 2020, 231 (03):
  • [16] Preparation of heterostructured TiO2/MoS2 for efficient photocatalytic rhodamine B degradation
    Li, Ping
    Gao, Mengyou
    Sun, Lei
    Xu, Huizhong
    Dong, Xiaochen
    Lin, Jianjian
    MATERIALS ADVANCES, 2022, 3 (04): : 2185 - 2190
  • [17] Surface Defect Engineering of MoS2 for Atomic Layer Deposition of TiO2 Films
    Kropp, Jaron A.
    Sharma, Ankit
    Zhu, Wenjuan
    Ataca, Can
    Gougousi, Theodosia
    ACS APPLIED MATERIALS & INTERFACES, 2020, 12 (42) : 48150 - 48160
  • [18] MoS2 Nanosheet Loaded with TiO2 Nanoparticles: An Efficient Electrocatalyst for Hydrogen Evolution Reaction
    Shen, Yongzhen
    Ren, Xiaohui
    Qi, Xiang
    Zhou, Jie
    Huang, Zongyu
    Zhong, Jianxin
    JOURNAL OF THE ELECTROCHEMICAL SOCIETY, 2016, 163 (13) : H1087 - H1090
  • [19] Efficient charge transfer on the tunable morphology of TiO2/MoS2 photocatalyst for an enhanced hydrogen production
    Gautam, Amit
    Prabhu, Yendrapati Taraka
    Pal, Ujjwal
    NEW JOURNAL OF CHEMISTRY, 2021, 45 (23) : 10257 - 10267
  • [20] RECONSTRUCTION OF TIO2(110) SURFACE - STM STUDY WITH ATOMIC-SCALE RESOLUTION
    ONISHI, H
    IWASAWA, Y
    SURFACE SCIENCE, 1994, 313 (1-2) : L783 - L789