Modulating H2 sorption in metal-organic frameworks via ordered functional groups

被引：10

作者：

Dau, Phuong V. ^{[1
]}

Cohen, Seth M. ^{[1
]}

机构：

[1] Univ Calif San Diego, Dept Chem & Biochem, La Jolla, CA 92093 USA

来源：

CHEMICAL COMMUNICATIONS | 2014年 / 50卷 / 81期

关键词：

HYDROGEN STORAGE; ADSORPTION; PORE;

D O I：

10.1039/c4cc05265j

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Herein, we present the use of presynthetic and postsynthetic modification (PSM) approaches to regulate the structural organization of functional groups in the pores of isoreticular metal-organic frameworks (IRMOFs). It has been found that the structural ordering of aryl groups within the IRMOF pores results in hysteretic H-2 sorption, while the same aryl groups introduced in a disordered manner displays reversible H-2 sorption that is more typical of the IRMOF family.

引用

页码：12154 / 12157

页数：4

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