Calculation of transient CIDEP spectra of spin-correlated radical pairs in nanotubes

被引：2
|
作者：
Lukzen, N. N.
Ivanov, K. L.
Morozov, V. A.
Kattnig, D. R.
Grampp, G.
机构：
[1] Int Tomog Ctr, Novosibirsk 630090, Russia
[2] Novosibirsk State Univ, Novosibirsk 630090, Russia
[3] Free Univ Berlin, D-14195 Berlin, Germany
[4] Graz Univ Technol, A-8010 Graz, Austria
来源：
CHEMICAL PHYSICS | 2006年 / 328卷 / 1-3期
基金：
俄罗斯基础研究基金会;
关键词：
CIDEP; EPR; nanochemistry; radical pairs;
D O I：
10.1016/j.chemphys.2006.06.014
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
The chemically induced dynamic electron polarization (CIDEP) formed by spin-correlated radical pairs in nanotubes is studied theoretically. Numerical solutions of the stochastic Liouville equation of the density operator are obtained by finite-difference methods. The nanotube is modelled as a one-dimensional nanoreactor with the relative motion of the radicals assumed to be free diffusion. The effect of the non-averaged dipole-dipole interaction of the electron spins on the CIDEP formation is studied in detail. Furthermore, the influence of the radical mobility and the nanotube orientation with respect to the external magnetic field are elucidated. (c) 2006 Elsevier B.V. All rights reserved.
引用
收藏
页码：75 / 84
页数：10
相关论文
共 50 条
  • [21] Influence of radical ion dimerization on spin dynamics of spin-correlated radical ion pairs
    Ivanov, K. L.
    DOKLADY PHYSICAL CHEMISTRY, 2006, 409 (1) : 210 - 213
  • [22] A manifestation of two-quantum transitions in the ODEPR spectra of the spin-correlated radical pairs in micelles
    Mursalimov, LR
    Salikhov, KM
    APPLIED MAGNETIC RESONANCE, 2001, 21 (02) : 223 - 248
  • [23] Features of the Primary Electron Spin Echo Signal for Spin-Correlated Radical Pairs
    Salikhov, K. M.
    Sukhanov, A. A.
    Khairutdinov, I. T.
    APPLIED MAGNETIC RESONANCE, 2024, 55 (04) : 463 - 475
  • [24] Features of the Primary Electron Spin Echo Signal for Spin-Correlated Radical Pairs
    K. M. Salikhov
    A. A. Sukhanov
    I. T. Khairutdinov
    Applied Magnetic Resonance, 2024, 55 : 463 - 475
  • [25] Organic photostimulated luminescence associated with persistent spin-correlated radical pairs
    Sakurai, Manabu
    Kabe, Ryota
    Fuki, Masaaki
    Lin, Zesen
    Jinnai, Kazuya
    Kobori, Yasuhiro
    Adachi, Chihaya
    Tachikawa, Takashi
    COMMUNICATIONS MATERIALS, 2021, 2 (01)
  • [26] Origin of Light-Induced Spin-Correlated Radical Pairs in Cryptochrome
    Weber, Stefan
    Biskup, Till
    Okafuji, Asako
    Marino, Anthony R.
    Berthold, Thomas
    Link, Gerhard
    Hitomi, Kenichi
    Getzoff, Elizabeth D.
    Schleicher, Erik
    Norris, James R., Jr.
    JOURNAL OF PHYSICAL CHEMISTRY B, 2010, 114 (45): : 14745 - 14754
  • [27] Comment on a shape of EPR spectra of spin-correlated radical pairs and separate radicals escaped geminate recombination
    K. M. Salikhov
    Applied Magnetic Resonance, 1997, 13 : 415 - 437
  • [28] Organic photostimulated luminescence associated with persistent spin-correlated radical pairs
    Manabu Sakurai
    Ryota Kabe
    Masaaki Fuki
    Zesen Lin
    Kazuya Jinnai
    Yasuhiro Kobori
    Chihaya Adachi
    Takashi Tachikawa
    Communications Materials, 2
  • [29] Zero Quantum Coherence in a Series of Covalent Spin-Correlated Radical Pairs
    Nelson, Jordan N.
    Krzyaniak, Matthew D.
    Horwitz, Noah E.
    Rugg, Brandon K.
    Phelan, Brian T.
    Wasielewski, Michael R.
    JOURNAL OF PHYSICAL CHEMISTRY A, 2017, 121 (11): : 2241 - 2252
  • [30] Comment on a shape of EPR spectra of spin-correlated radical pairs and separate radicals escaped geminate recombination
    Salikhov, KM
    APPLIED MAGNETIC RESONANCE, 1997, 13 (3-4) : 415 - 437
12345