The Spider DMA: A miniature radial differential mobility analyzer

被引:5
|
作者
Amanatidis, Stavros [1 ]
Kim, Changhyuk [1 ,2 ]
Spielman, Steven R. [3 ]
Lewis, Gregory S. [3 ]
Hering, Susanne, V [3 ]
Flagan, Richard C. [1 ]
机构
[1] CALTECH, Div Chem & Chem Engn, Pasadena, CA 91125 USA
[2] Pusan Natl Univ, Dept Environm Engn, Busan, South Korea
[3] Aerosol Dynam Inc, Berkeley, CA USA
关键词
Jingkun Jiang; SPECTROMETER; PERFORMANCE; RESOLUTION; DESIGN;
D O I
10.1080/02786826.2019.1626974
中图分类号
TQ [化学工业];
学科分类号
0817 ;
摘要
The Spider differential mobility analyzer (DMA) is a novel, miniaturized radial DMA developed to provide size classification in the 10-500 nm range for applications requiring high portability and time resolution. Its external dimensions are similar to 12 cm in diameter by 6 cm in height (excluding tubing); it weighs similar to 350 g, and is designed to operate at 0.6-1.5 L/min sheath and 0.3 L/min sample flowrates. It features a new sample inlet geometry that is designed to produce a uniform azimuthal particle distribution at the entrance of the classifier, optimized sample/sheath flow streams introduction in the classifier to minimize particle delays, and extension of the electric field interaction volume for similar to 30% enhanced dynamic range. Based on three-dimensional finite element simulations of flows, electric fields, and particle trajectories, we demonstrate that the Spider DMA transfer functions can be predicted with high fidelity using a parameterized fit based on the Stolzenburg semi-analytical model. Experimental characterization of the instrument response with size-selected particles confirmed close agreement with model prediction; mobility size response is linear over three orders of magnitude in mobility span. Electrical ground shielding of the external surfaces of the DMA has been found to be necessary to avoid particle losses associated with field effects as the high voltage operating limit is approached. The mean deviation between the reference size of polystyrene latex spheres and the Spider DMA measurement is less than 2%, corroborating its high sizing precision and potential for high quality size distribution measurements. Copyright (c) 2019 American Association for Aerosol Research
引用
收藏
页码:175 / 189
页数:15
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