Enhanced photovoltaic performance of perovskite CH3NH3PbI3 solar cells with freestanding TiO2 nanotube array films

被引:152
|
作者
Gao, Xianfeng [1 ]
Li, Jianyang [1 ]
Baker, Joel [1 ]
Hou, Yang [1 ]
Guan, Dongsheng [1 ]
Chen, Junhong [1 ]
Yuan, Chris [1 ]
机构
[1] Univ Wisconsin, Dept Mech Engn, Milwaukee, WI 53211 USA
基金
美国国家科学基金会;
关键词
EFFICIENCY; TRANSPORT;
D O I
10.1039/c4cc01864h
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Freestanding TiO2 nanotube array films are fabricated and first applied as electrodes in perovskite CH3NH3PbI3 sensitized solar cells. The device demonstrates improved light absorption with more than 90% of light absorbed in the whole visible range and a reduced charge recombination rate, leading to a significant improvement of the photocurrent and efficiency. This study suggests a promising way of improving the conversion efficiency of perovskite solar cells through novel electrodes.
引用
收藏
页码:6368 / 6371
页数:4
相关论文
共 50 条
  • [41] Credible evidence for the passivation effect of remnant PbI2 in CH3NH3PbI3 films in improving the performance of perovskite solar cells
    Wang, Shimao
    Dong, Weiwei
    Fang, Xiaodong
    Zhang, Qingli
    Zhou, Shu
    Deng, Zanhong
    Tao, Ruhua
    Shao, Jingzhen
    Xia, Rui
    Song, Chao
    Hu, Linhua
    Zhu, Jun
    NANOSCALE, 2016, 8 (12) : 6600 - 6608
  • [42] Controlled crystallization of CH3NH3PbI3 filmS for perovskite solar cells by various PbI2(X) complexes
    Fu, Weifei
    Yan, Jielin
    Zhang, Zhongqiang
    Ye, Tao
    Liu, Yujing
    Wu, Jiake
    Yao, Jizhong
    Li, Chang-Zhi
    Li, Hanying
    Chen, Hongzheng
    SOLAR ENERGY MATERIALS AND SOLAR CELLS, 2016, 155 : 331 - 340
  • [43] Cooperative kinetics of depolarization in CH3NH3PbI3 perovskite solar cells
    Bertoluzzi, Luca
    Sanchez, Rafael S.
    Liu, Linfeng
    Lee, Jin-Wook
    Mas-Marza, Elena
    Han, Hongwei
    Park, Nam-Gyu
    Mora-Sero, Ivan
    Bisquert, Juan
    ENERGY & ENVIRONMENTAL SCIENCE, 2015, 8 (03) : 910 - 915
  • [44] Opportunities of copper addition in CH3NH3PbI3 perovskite and their photovoltaic performance evaluation
    Khalid, Maria
    Roy, Anurag
    Bhandari, Shubhranshu
    Selvaraj, Prabhakaran
    Sundaram, Senthilarasu
    Mallick, Tapas K.
    JOURNAL OF ALLOYS AND COMPOUNDS, 2022, 895
  • [45] First-Principles Study of Electron Injection and Defects at the TiO2/CH3NH3PbI3 Interface of Perovskite Solar Cells
    Haruyama, Jun
    Sodeyama, Keitaro
    Hamada, Ikutaro
    Han, Liyuan
    Tateyama, Yoshitaka
    JOURNAL OF PHYSICAL CHEMISTRY LETTERS, 2017, 8 (23): : 5840 - 5847
  • [46] Fabrication of perovskite solar cells using sputter-processed CH3NH3PbI3 films
    Raifuku, Itaru
    Ishikawa, Yasuaki
    Bourgeteau, Tiphaine
    Bonnassieux, Yvan
    Roca i Cabarrocas, Pere
    Uraoka, Yukiharu
    APPLIED PHYSICS EXPRESS, 2017, 10 (09)
  • [47] Morphological improvement of CH3NH3PbI3 films using blended solvents for perovskite solar cells
    Nam Le
    Nguyen Tam Nguyen Truong
    Trang Le
    Mohan Reddy Pallavolu
    Hye Jun Jeon
    Chinho Park
    Korean Journal of Chemical Engineering, 2021, 38 : 187 - 194
  • [48] Enhancing the photocurrent of perovskite solar cells via modification of the TiO2/CH3NH3PbI3 heterojunction interface with amino acid
    Shih, Y. C.
    Wang, L. Y.
    Hsieh, H. C.
    Lin, K. F.
    JOURNAL OF MATERIALS CHEMISTRY A, 2015, 3 (17) : 9133 - 9136
  • [49] Stabilizing TiO2/CH3NH3PbI3 heterostructure and enhancing interface trap passivation for efficient and stable perovskite solar cells
    Xu, Shendong
    Liang, Zheng
    Zheng, Haiying
    Zhang, Liying
    Xu, Xiaoxiao
    Xu, Huifen
    Zhu, Liangzheng
    Ye, Jiajiu
    Liu, Guozhen
    Pan, Xu
    JOURNAL OF MATERIALS CHEMISTRY C, 2021, 9 (31) : 9982 - 9989
  • [50] Study on light absorption of CH3NH3PbI3 perovskite solar cells enhanced by gold nanobipyramids
    Chen, Le
    Luo, Wei
    Fang, Bowen
    Zhu, Baohua
    Zhang, Wentao
    OPTICS AND LASER TECHNOLOGY, 2023, 159