Noncontact atomic force microscopy imaging of water dissociation products on TiO2(110)

被引:42
|
作者
Pang, C. L. [1 ]
Sasahara, A.
Onishi, H.
Chen, Q.
Thornton, G.
机构
[1] Kobe Univ, Fac Sci, Dept Chem, Kobe, Hyogo 6578501, Japan
[2] Japan Sci & Technol Agcy, Kawaguchi, Saitama 3320012, Japan
[3] UCL, London Ctr Nanotechnol, London WC1H 0AJ, England
[4] UCL, Dept Chem, London WC1H 0AJ, England
来源
PHYSICAL REVIEW B | 2006年 / 74卷 / 07期
关键词
D O I
10.1103/PhysRevB.74.073411
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
We have imaged the products of water dissociation on TiO(2)(110) with noncontact atomic force microscopy (NC-AFM). Scanning tunneling microscopy (STM) experiments have revealed that water splits into a hydroxyl group that sits in an O vacancy and an H adatom which lies on a bridging O atom. With this knowledge, STM images acquired in the same area allow an unambiguous identification of these H adatoms in the corresponding NC-AFM images.
引用
收藏
页数:4
相关论文
共 50 条
  • [21] Fluctuation of acetate ions in the (2 x 1)-acetate overlayer on TiO2(110)-(1 x 1) observed by noncontact atomic force microscopy
    Fukui, K
    Iwasawa, Y
    SURFACE SCIENCE, 2000, 464 (2-3) : L719 - L726
  • [22] Imaging of individual formate ions adsorbed on TiO2(110) surface by non-contact atomic force microscopy
    Fukui, K
    Onishi, H
    Iwasawa, Y
    CHEMICAL PHYSICS LETTERS, 1997, 280 (3-4) : 296 - 301
  • [23] Atomic resolution noncontact atomic force and scanning tunneling microscopy of TiO2(110)-(1x1) and -(1x2):: Simultaneous imaging of surface structures and electronic states
    Ashino, M
    Sugawara, Y
    Morita, S
    Ishikawa, M
    PHYSICAL REVIEW LETTERS, 2001, 86 (19) : 4334 - 4337
  • [24] Noncontact atomic force microscopy: Bond imaging and beyond
    Zhong, Qigang
    Li, Xuechao
    Zhang, Haiming
    Chi, Lifeng
    SURFACE SCIENCE REPORTS, 2020, 75 (04)
  • [25] Ab Initio Modeling of Noncontact Atomic Force Microscopy Imaging of Benzene on Cu(110) Surface
    Atodiresei, N.
    Caciuc, V.
    Hoelscher, H.
    Bluegel, S.
    INTERNATIONAL JOURNAL OF QUANTUM CHEMISTRY, 2008, 108 (15) : 2803 - 2812
  • [26] Atomic force microscopy images of MgO(100) and TiO2(110) under water and aqueous aromatic molecule solutions
    Komiyama, M
    Gu, MM
    APPLIED SURFACE SCIENCE, 1997, 120 (1-2) : 125 - 128
  • [27] Atomic Scale Imaging of TiO2(100) Reconstructed Surfaces by Noncontact Scanning Nonlinear Dielectric Microscopy
    Sawai, Nobuhiro
    Yamasue, Kohei
    Cho, Yasuo
    JAPANESE JOURNAL OF APPLIED PHYSICS, 2012, 51 (12)
  • [28] Frequency modulation atomic force microscope observation of TiO2(110) surfaces in water
    Sasahara, Akira
    Tomitori, Masahiko
    JOURNAL OF VACUUM SCIENCE & TECHNOLOGY B, 2010, 28 (03):
  • [29] Imaging water dissociation on TiO2(110):: Evidence for inequivalent geminate OH groups
    Zhang, Z.
    Bondarchuk, O.
    Kay, Bruce D.
    White, J. M.
    Dohnalek, Z.
    JOURNAL OF PHYSICAL CHEMISTRY B, 2006, 110 (43): : 21840 - 21845
  • [30] Atomic-resolution imaging of rutile TiO2(110)-(1 x 2) reconstructed surface by non-contact atomic force microscopy
    Katsube D.
    Ojima S.
    Inami E.
    Abe M.
    Beilstein Journal of Nanotechnology, 2020, 11 : 443 - 449