Intensity dependence of the dissociative ionization of DCl in few-cycle laser fields

被引:11
|
作者
Li, H. [1 ,2 ]
Tong, X. M. [3 ,4 ]
Schirmel, N. [5 ]
Urbasch, G. [5 ]
Betsch, K. J. [1 ]
Zherebtsov, S. [1 ]
Suessmann, F. [1 ]
Kessel, A. [1 ]
Trushin, S. A. [1 ]
Paulus, G. G. [6 ,7 ]
Weitzel, K-M [5 ]
Kling, M. F. [1 ,2 ]
机构
[1] Max Planck Inst Quantum Opt, D-85748 Garching, Germany
[2] Univ Munich, Fak Phys, D-85748 Garching, Germany
[3] Univ Tsukuba, Inst Mat Sci, Tsukuba, Ibaraki 3058573, Japan
[4] Univ Tsukuba, Ctr Computat Sci, Tsukuba, Ibaraki 3058577, Japan
[5] Univ Marburg, Fachbereich Chem, D-35032 Marburg, Germany
[6] Univ Jena, Inst Opt & Quantenelekt, D-07743 Jena, Germany
[7] Helmholtz Inst Jena, D-07743 Jena, Germany
基金
日本学术振兴会;
关键词
CEP control; attosecond physics; molecular dynamics; ENVELOPE-PHASE DEPENDENCE; ELECTRON LOCALIZATION; MOLECULES; BOND;
D O I
10.1088/0953-4075/49/1/015601
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
We have studied the dissociative ionization of DCl in 4 fs laser fields at 720 nm central wavelength using intensities in the range (1.3-3.1) x 10(14) W cm(-2). By employing the phase-tagged velocity-map imaging technique, information about the angular distribution of deuterium ions as a function of their kinetic energy and the carrier-envelope phase is obtained. On the basis of the experimental data and semi-classical simulations, three regions are distinguished for the resulting D+ ions with different kinetic energies. The one with the lowest kinetic energy, around 5-7 eV, is from dissociation involving the X-state of DCl+, populated through direct ionization with the laser field. The second region, around 7-11 eV, originates from rescattering induced dissociative ionization. Above 2 x 10(14) W cm(-2) D+ ions with kinetic energies exceeding 15 eV are obtained, which we ascribe to double ionization induced by rescattered electrons.
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页数:8
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