Spectral Control of an X-Ray L-Edge Transition via a Thin-Film Cavity

被引:21
|
作者
Haber, Johann [1 ]
Gollwitzer, Jakob [1 ]
Francoual, Sonia [1 ]
Tolkiehn, Martin [1 ]
Strempfer, Joerg [1 ]
Roehlsberger, Ralf [1 ,2 ]
机构
[1] DESY, Notkestr 85, D-22607 Hamburg, Germany
[2] Hamburg Ctr Ultrafast Imaging, Luruper Chaussee 149, D-22761 Hamburg, Germany
关键词
LAMB SHIFT; QUANTUM-ELECTRODYNAMICS; ATOMS; STATES; RADIATION; NUCLEI; LINES;
D O I
10.1103/PhysRevLett.122.123608
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
By embedding a thin layer of tantalum in an x-ray cavity, we observe a change in the spectral characteristics of an inner-shell transition of the metal. The interaction between the cavity mode vacuum and the L-m-edge transition is enhanced, permitting the observation of the collective Lamb shift, superradiance, and a Fano-like cavity-resonance interference effect. This experiment demonstrates the feasibility of cavity quantum electrodynamics with electronic resonances in the x-ray range with applications to manipulating and probing the electronic structure of condensed matter with high-resolution x-ray spectroscopy in an x-ray cavity setting.
引用
收藏
页数:5
相关论文
共 50 条
  • [41] Investigation of thickness dependence on electronic structures of iron and nickel thin films by L-edge X-ray absorption spectroscopy
    Akgul, Guvenc
    Akgul, Funda Aksoy
    Ufuktepe, Yuksel
    VACUUM, 2014, 99 : 211 - 215
  • [42] Sum rules of L-edge x-ray magnetic circularly polarized emission for 3d transition metals
    Koide, Akihiro
    Nomura, Takuji
    Inami, Toshiya
    PHYSICAL REVIEW B, 2021, 104 (09)
  • [43] 3d transition metal L-edge X-ray absorption studies of the dichalcogenides of Fe, Co and Ni
    Charnock, JM
    Henderson, CMB
    Mosselmans, JFW
    Pattrick, RAD
    PHYSICS AND CHEMISTRY OF MINERALS, 1996, 23 (07) : 403 - 408
  • [44] Theory of Cu L-edge resonant inelastic X-ray scattering in insulating cuprates
    Tsutsui, K
    Yamamoto, H
    Tohyama, T
    Maekawa, S
    JOURNAL OF PHYSICS AND CHEMISTRY OF SOLIDS, 2006, 67 (1-3) : 274 - 276
  • [45] Unraveling the Electronic Structure of Photocatalytic Manganese Complexes by L-Edge X-ray Spectroscopy
    Bokarev, Sergey I.
    Khan, Munirah
    Abdel-Latif, Mahmoud K.
    Xiao, Jie
    Hila, Rifaat
    Aziz, Saadullah G.
    Aziz, Emad F.
    Kuehn, Oliver
    JOURNAL OF PHYSICAL CHEMISTRY C, 2015, 119 (33): : 19192 - 19200
  • [46] X-ray-induced sample damage at the Mn L-edge: a case study for soft X-ray spectroscopy of transition metal complexes in solution
    Kubin, Markus
    Kern, Jan
    Guo, Meiyuan
    Kallman, Erik
    Mitzner, Rolf
    Yachandra, Vittal K.
    Lundberg, Marcus
    Yano, Junko
    Wernet, Philippe
    PHYSICAL CHEMISTRY CHEMICAL PHYSICS, 2018, 20 (24) : 16817 - 16827
  • [47] STUDY OF THE TRANSMISSION OF MULTILAYERED THIN-FILM X-RAY GUIDES
    DUDCHIK, YI
    KOMAROV, FF
    KUMAKHOV, MA
    LOBOTSKII, DG
    SOLOVEV, VS
    TISHKOV, VS
    PISMA V ZHURNAL TEKHNICHESKOI FIZIKI, 1991, 17 (13): : 82 - 86
  • [48] A STUDY OF TRANSMISSION OF MULTILAYER THIN-FILM X-RAY GUIDES
    DUDCHIK, YI
    KOMAROV, FF
    LOBOTSKY, DG
    SOLOVIEV, VS
    TISHKOV, VS
    NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT, 1993, 325 (1-2): : 343 - 345
  • [49] X-RAY PHOTOACOUSTIC-SPECTROSCOPY OF ZNO THIN-FILM
    TOYODA, T
    MASUJIMA, T
    ANDO, M
    JAPANESE JOURNAL OF APPLIED PHYSICS PART 1-REGULAR PAPERS SHORT NOTES & REVIEW PAPERS, 1993, 32 (5B): : 2550 - 2553
  • [50] Study of transmission of multilayer thin-film X-ray guides
    Dudchik, Yu.I.
    Komarov, F.F.
    Lobotsky, D.G.
    Soloviev, V.S.
    Tishkov, V.S.
    Nuclear Instruments and Methods in Physics Research, Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, 1993, A325 (1-2) : 343 - 345