Room-Temperature Giant Persistent Photoconductivity in SrTiO3/LaAlO3 Heterostructures

被引:141
|
作者
Tebano, Antonello [1 ,2 ]
Fabbri, Emiliana [3 ]
Pergolesi, Daniele [3 ]
Balestrino, Giuseppe [1 ,2 ]
Traversa, Enrico [3 ]
机构
[1] Univ Roma Tor Vergata, CNR SPIN, Rome, Italy
[2] Univ Roma Tor Vergata, Dipartimento Informat Sistemi & Prod, Rome, Italy
[3] Natl Inst Mat Sci, Int Res Ctr Mat Nanoarchitecton MANA, Tsukuba, Ibaraki, Japan
关键词
SrTiO3/LaAlO3; interfaces; persistent photocurrent; electrochemical impedance spectroscopy; ELECTRON-GAS; INTERFACES;
D O I
10.1021/nn203991q
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
SrTiO3/LaAlO3 interfaces show an unprecedented photoconductivity effect that is persistent even at room temperature and giant as It gives rise to a conductivity increase of about 5 orders of magnitude at room temperature. The persistent photoconductivity effects play a paramount role in the still controversial intrinsic behavior of the SrTiO3/LaAlO3 interfaces, as even a limited exposure to visible light is able to strongly modify the electrical transport properties of the interface even above room temperature, while only an appropriate thermal treatment in a dark environment can completely suppress the persistent photoconductivity effect unveiling the intrinsic conduction mechanism of the interface. Moreover, our study demonstrates that the origin of the high conductivity, revealed at the STO/LAO Interface at room temperature, is purely electronic.
引用
收藏
页码:1278 / 1283
页数:6
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