Incommensurate magnetic ground state revealed by resonant x-ray scattering in the frustrated spin system Ca3Co2O6

被引:71
|
作者
Agrestini, S. [1 ]
Mazzoli, C. [2 ]
Bombardi, A. [3 ]
Lees, M. R. [1 ]
机构
[1] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England
[2] European Synchrotron Radiat Facil, F-38043 Grenoble, France
[3] Rutherford Appleton Lab, Diamond Light Source Ltd, Didcot OX11 0QX, Oxon, England
来源
PHYSICAL REVIEW B | 2008年 / 77卷 / 14期
关键词
D O I
10.1103/PhysRevB.77.140403
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
We have performed a resonant x-ray scattering study at the Co pre-K edge on a single crystal of Ca(3)Co(2)O(6). The measurements reveal an abrupt transition to a magnetically ordered state immediately below T(N)=25 K, with a magnetic correlation length in excess of 5500 A along the c axis chains. There is no evidence for modifications to the Co(3+) spin state. A temperature dependent modulation in the magnetic order along the c axis and an unusual decrease in the magnetic correlation lengths on cooling are observed. The results are compatible with the onset of a partially disordered antiferromagnetic structure in Ca(3)Co(2)O(6).
引用
收藏
页数:4
相关论文
共 50 条
  • [21] Formation of Magnetic Microphases in Ca3Co2O6
    Kamiya, Y.
    Batista, C. D.
    PHYSICAL REVIEW LETTERS, 2012, 109 (06)
  • [22] Dielectric anomalies and magnetodielectric coupling behavior of single crystalline Ca3Co2O6, a geometrically frustrated magnetic spin-chain system
    Basu, Tathamay
    Iyer, Kartik K.
    Paulose, P.L.
    Sampathkumaran, E.V.
    Journal of Alloys and Compounds, 2016, 675 : 364 - 369
  • [23] Specific heat investigation of the magnetic ordering in two frustrated spin-chain oxides:: Ca3Co2O6 and Ca3CoRhO6
    Hardy, V
    Lees, MR
    Maignan, A
    Hébert, S
    Flahaut, D
    Martin, C
    Paul, DM
    JOURNAL OF PHYSICS-CONDENSED MATTER, 2003, 15 (33) : 5737 - 5746
  • [24] Nature of the magnetic order in Ca3Co2O6
    Agrestini, S.
    Chapon, L. C.
    Daoud-Aladine, A.
    Schefer, J.
    Gukasov, A.
    Mazzoli, C.
    Lees, M. R.
    Petrenko, O. A.
    PHYSICAL REVIEW LETTERS, 2008, 101 (09)
  • [25] Spin-Orbit-Lattice Entangled State in A2MgReO6 (A = Ca, Sr, Ba) Revealed by Resonant Inelastic X-Ray Scattering
    Frontini, Felix I.
    Johnstone, Graham H. J.
    Iwahara, Naoya
    Bhattacharyya, Pritam
    Bogdanov, Nikolay A.
    Hozoi, Liviu
    Upton, Mary H.
    Casa, Diego M.
    Hirai, Daigorou
    Kim, Young-June
    PHYSICAL REVIEW LETTERS, 2024, 133 (03)
  • [26] Metastable states in the frustrated triangular compounds Ca3Co2-xMnxO6 and Ca3Co2O6
    Kim, Jae Wook
    Mun, E. D.
    Ding, X.
    Hansen, A.
    Jaime, M.
    Harrison, N.
    Yi, H. T.
    Chai, Y.
    Sun, Y.
    Cheong, S. W.
    Zapf, V. S.
    PHYSICAL REVIEW B, 2018, 98 (02)
  • [27] Effects of Ho-ion substitution on the magnetic properties of the Ca3Co2O6 frustrated spin-chain compound
    Gong, Gaoshang
    Wang, Yongqiang
    Su, Yuling
    Liu, Dewei
    Zerihun, Gebru
    Qiu, Yang
    MATERIALS RESEARCH BULLETIN, 2018, 99 : 419 - 423
  • [28] Synthesis of fine particles of a geometrically frustrated spin-chain system Ca3Co2O6 through a pyrophoric route and its magnetic behavior
    Mukherjee, K.
    Sampathkumaran, E. V.
    JOURNAL OF ALLOYS AND COMPOUNDS, 2010, 498 (01) : 1 - 4
  • [29] Long-time variation of magnetic structure in a geometrically frustrated magnet Ca3Co2O6
    Moyoshi, Taketo
    Takahashi, Rui
    Motoya, Kiyoichiro
    INTERNATIONAL CONFERENCE ON STRONGLY CORRELATED ELECTRON SYSTEMS (SCES 2010), 2011, 273
  • [30] Microscopic derivation of magnetic coupling in Ca3Co2O6
    Laschinger, C
    Kopp, T
    Eyert, V
    Frésard, R
    JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS, 2004, 272 : 974 - 975