Fast response photogating in monolayer MoS2 phototransistors

被引:21
|
作者
Vaquero, Daniel [1 ]
Clerico, Vito [1 ]
Salvador-Sanchez, Juan [1 ]
Diaz, Elena [2 ]
Dominguez-Adame, Francisco [2 ]
Chico, Leonor [2 ,3 ]
Meziani, Yahya M. [1 ]
Diez, Enrique [1 ]
Quereda, Jorge [1 ]
机构
[1] Univ Salamanca, USAL Nanolab, Nanotechnol Grp, E-37008 Salamanca, Spain
[2] Univ Complutense, Dept Fis Mat, GISC, E-28040 Madrid, Spain
[3] CSIC, Inst Ciencia Mat Madrid, E-28049 Madrid, Spain
关键词
MECHANISMS; GAIN;
D O I
10.1039/d1nr03896f
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Two-dimensional transition metal dichalcogenide (TMD) phototransistors have been the object of intensive research during the last years due to their potential for photodetection. Photoresponse in these devices is typically caused by a combination of two physical mechanisms: the photoconductive effect (PCE) and photogating effect (PGE). In earlier literature for monolayer (1L) MoS2 phototransistors, PGE is generally attributed to charge trapping by polar molecules adsorbed to the semiconductor channel, giving rise to a very slow photoresponse. Thus, the photoresponse of 1L-MoS2 phototransistors at high-frequency light modulation is assigned to PCE alone. Here we investigate the photoresponse of a fully h-BN encapsulated monolayer (1L) MoS2 phototransistor. In contrast with previous understanding, we identify a rapidly-responding PGE mechanism that becomes the dominant contribution to photoresponse under high-frequency light modulation. Using a Hornbeck-Haynes model for the photocarrier dynamics, we fit the illumination power dependence of this PGE and estimate the energy level of the involved traps. The resulting energies are compatible with shallow traps in MoS2 caused by the presence of sulfur vacancies.
引用
收藏
页码:16156 / 16163
页数:8
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