Transient multi pulse method for the determination of N2O -: Interaction with ZSM-5 type zeolites

被引:10
|
作者
Ates, A
Reitzmann, A
机构
[1] Univ Karlsruhe, Inst Chem Verfahrenstech, D-76128 Karlsruhe, Germany
[2] Cumhuriyet Univ, Dept Chem Engn, TR-58000 Sivas, Turkey
来源
关键词
nitrous oxide; zeolite; surface oxygen; transient method;
D O I
10.1007/s11144-005-0289-z
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Multipulse experiments reveal qualitative and quantitative, time-resolved information about the interaction of N2O with ZSM-5 type zeolites under conditions of catalytic applications, like the mechanism of N2O decomposition, amount and reactivity of an atomic surface oxygen species.
引用
收藏
页码:11 / 20
页数:10
相关论文
共 50 条
  • [41] Role of aggregated Fe oxo species in N2O decomposition over Fe/ZSM-5
    Zhang, Bo
    Liu, Fudong
    He, Hong
    Xue, Li
    CHINESE JOURNAL OF CATALYSIS, 2014, 35 (12) : 1972 - 1981
  • [42] Enhancement of α-oxygen formation and N2O decomposition on Fe/ZSM-5 catalysts by extraframework Al
    Sun, KQ
    Zhang, HD
    Xia, H
    Lian, YX
    Li, Y
    Feng, ZC
    Ying, PL
    Li, C
    CHEMICAL COMMUNICATIONS, 2004, (21) : 2480 - 2481
  • [43] Catalytic properties of extraframework iron-containing species in ZSM-5 for N2O decomposition
    Li, Guanna
    Pidko, Evgeny A.
    Filot, Ivo A. W.
    van Santen, Rutger A.
    Li, Can
    Hensen, Emie J. M.
    JOURNAL OF CATALYSIS, 2013, 308 : 386 - 397
  • [44] Role of Al pairs on effective N2O decomposition over the ZSM-5 zeolite catalyst
    Kang, Bin
    Li, Ming
    Di, Zhaoying
    Guo, Xiaonan
    Wei, Ying
    Jia, Jingbo
    Zhang, Runduo
    CATALYSIS TODAY, 2022, 402 : 17 - 26
  • [45] PROPERTIES OF ZSM-5 TYPE ZEOLITES RELATED TO THE SIO2/AL2O3 RATIO
    BERAK, JM
    KANIK, B
    EYSYMONTT, P
    MEJSNER, J
    REACTION KINETICS AND CATALYSIS LETTERS, 1984, 25 (3-4): : 323 - 327
  • [46] Density Functional Calculations on the Adsorption of N2O and H2O on the Ion-exchanged ZSM-5
    Gao, H. W.
    Guo, L.
    Deng, H. H.
    Ge, L. Y.
    Yan, T. X.
    POLISH JOURNAL OF CHEMISTRY, 2009, 83 (06) : 1195 - 1201
  • [47] Theoretical study of N2O decomposition mechanism over binuclear Cu-ZSM-5 zeolites
    Liu, Xin
    Yang, Zuoyin
    Li, Yaping
    Zhang, Fazhi
    Journal of Molecular Catalysis A: Chemical, 2015, 396 : 181 - 187
  • [48] Theoretical study of N2O decomposition mechanism over binuclear Cu-ZSM-5 zeolites
    Liu, Xin
    Yang, Zuoyin
    Li, Yaping
    Zhang, Fazhi
    JOURNAL OF MOLECULAR CATALYSIS A-CHEMICAL, 2015, 396 : 181 - 187
  • [49] Photocatalytic decomposition of N2O into N2 and O2 on the silver(I) ion-exchanged ZSM-5 catalyst
    Matsuoka, M
    Ju, WS
    Anpo, M
    CHEMISTRY LETTERS, 2000, (06) : 626 - 627
  • [50] A transient kinetic study of the oscillating N2O decomposition over Cu-ZSM-5
    Turek, T
    JOURNAL OF CATALYSIS, 1998, 174 (01) : 98 - 108