Odd electron wave packets from cycloidal ultrashort laser fields

被引:46
|
作者
Kerbstadt, S. [1 ]
Eickhoff, K. [1 ]
Bayer, T. [1 ]
Wollenhaupt, M. [1 ]
机构
[1] Carl von Ossietzky Univ Oldenburg, Inst Phys, Carl von Ossietzky Str 9-11, D-26129 Oldenburg, Germany
关键词
POLARIZATION; MOMENTUM;
D O I
10.1038/s41467-019-08601-7
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
Polarization-tailored bichromatic femtosecond laser fields with cycloidal polarization profiles have emerged as a powerful tool for coherent control of quantum processes. We present an optical scheme to create and manipulate three-dimensional free electron wave packets with arbitrary rotational symmetry by combining advanced supercontinuum pulse shaping with high resolution photoelectron tomography. Here we use carrier-envelope phase-stable polarization-tailored bichromatic (3 omega:4 omega) counter- and corotating femtosecond laser pulses to generate 7-fold rotational symmetric and asymmetric photoelectron momentum distributions by multiphoton ionization of sodium atoms. To elucidate the physical mechanisms, we investigate the interplay between the symmetry properties of the driving field and the resulting electron wave packets by varying the optical field parameters. Our results show that the symmetry properties of electron wave packets are not fully determined by the field symmetry, but completely described by multipath quantum interference of states with different angular momenta.
引用
收藏
页数:8
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