TiO2 nanoparticles and CQDs co-decorated mesoporous g-C3N4 and their photocatalytic properties for gaseous benzene degradation

被引:6
|
作者
Zhao, Chunxia [1 ]
Jia, Heng [1 ]
Jin, Wei [2 ]
Li, Feng [1 ]
Li, Hang [1 ]
Chen, Wen [1 ]
机构
[1] Wuhan Univ Technol, Sch Mat Sci & Engn, State Key Lab Adv Technol Mat Synth & Proc, Wuhan 430070, Hubei, Peoples R China
[2] Wuhan Univ Technol, State Key Lab Silicate Mat Architectures, Wuhan 430070, Hubei, Peoples R China
基金
国家重点研发计划;
关键词
Mesoporous g-C3N4; TiO2; nanoparticles; carbon quantum dots; photocatalysis; gaseous benzene; IN-SITU SYNTHESIS; CARBON-DOTS; ULTRATHIN NANOSHEETS; HETEROJUNCTIONS; NANOCOMPOSITE; FABRICATION; NITRIDE;
D O I
10.1142/S1793604719500863
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
Mesoporous g-C3N4 is prepared by a hard template method and is then decorated by carbon quantum dots (CQDs) and TiO2 nanoparticles through an impregnation route followed by a hydrothermal method. The synthesized hybrids possess higher specific surface area up to 131 cm(2)/g and show effective absorption of visible light range and improved instantaneous photocurrent response, which reveals the enhanced photo-generated carrier separation efficiency. The first-order kinetic reaction rate constant of photocatalytic degradation of gaseous benzene by TCPCN-2 is 5.5 times of the bulk g-C3N4. Its degradation rate is up to 96.08% with good photocatalytic stability. Thus, the TiO2 nanoparticles and CQDs co-decorated g-C3N4 hybrids are promising photocatalysts.
引用
收藏
页数:5
相关论文
共 50 条
  • [21] MOF-Derived Mesoporous g-C3N4/TiO2 Heterojunction with Enhanced Photocatalytic Activity
    Wei, Congcong
    Zhang, Wei
    Wang, Xinpeng
    Li, Aihong
    Guo, Jianping
    Liu, Bo
    CATALYSIS LETTERS, 2021, 151 (07) : 1961 - 1975
  • [22] 2D/2D g-C3N4/(001)-TiO2 Z-scheme heterojunction decorated with CQDs for enhanced Photocatalytic activity
    Wang, Yueying
    Chen, Jin
    Yang, Xiaofeng
    Liu, Xinwei
    Que, Meidan
    Ma, Yuzhao
    Li, Yanjun
    MATERIALS TODAY COMMUNICATIONS, 2023, 37
  • [23] Analysis of Photocatalytic Properties of NS-CQDs/g-C3N4 Composites
    Wang, Yu
    Chen, Hongyue
    Jia, Zijian
    Lv, Jingxue
    Lv, Yuguang
    Wu, Jiang
    MICROMACHINES, 2023, 14 (12)
  • [24] The effects of cotton cellulose on both energy band gap of g-C3N4–TiO2 nanoparticles and enhanced photocatalytic properties of cotton-g-C3N4–TiO2 composites
    Wenjun Li
    Hui Zhang
    Wendou Chen
    Limeng Yang
    Hailiang Wu
    Ningtao Mao
    Cellulose, 2022, 29 : 193 - 212
  • [25] TiO2 modified g-C3N4 with enhanced photocatalytic CO2 reduction performance
    Wang, Huiqin
    Li, Hongda
    Chen, Zhuowen
    Li, Jinze
    Li, Xin
    Huo, Pengwei
    Wang, Qian
    SOLID STATE SCIENCES, 2020, 100
  • [26] g-C3N4/TiO2 NANOCOMPOSITES AND THEIR APPLICATION IN PHOTOCATALYTIC CO2 REDUCTION: A MINIREVIEW
    Manrique-Holguin, M.
    Alvear-Daza, J. J.
    Rengifo-Herrera, J. A.
    Pizzio, L. R.
    LATIN AMERICAN APPLIED RESEARCH, 2023, 53 (01) : 71 - 76
  • [27] Ag2CO3 nanoparticles decorated g-C3N4 as a high-efficiency catalyst for photocatalytic degradation of organic contaminants
    Pan, Shugang
    Jia, Bingquan
    Fu, Yongsheng
    JOURNAL OF MATERIALS SCIENCE-MATERIALS IN ELECTRONICS, 2021, 32 (11) : 14464 - 14476
  • [28] Ag2CO3 nanoparticles decorated g-C3N4 as a high-efficiency catalyst for photocatalytic degradation of organic contaminants
    Shugang Pan
    Bingquan Jia
    Yongsheng Fu
    Journal of Materials Science: Materials in Electronics, 2021, 32 : 14464 - 14476
  • [29] Construction of (001)-TiO2/g-C3N4 heterojunction for enhanced photocatalytic degradation of methylene blue
    Gao, Ran
    Lin, Wensong
    Lin, Huanxia
    He, Yong
    Mai, Xin
    Zhang, Yeheng
    REACTION KINETICS MECHANISMS AND CATALYSIS, 2025, 138 (01) : 455 - 469
  • [30] Effect of Contact Mode of TiO2/g-C3N4 Heterojunction on Photocatalytic Performance for Dye Degradation
    Deng, Zijian
    Osuga, Ryota
    Matsubara, Masaki
    Kanie, Kiyoshi
    Muramatsu, Atsushi
    MATERIALS TRANSACTIONS, 2023, 64 (12) : 2782 - 2791