Morphological Engineering of Sensing Materials for Flexible Pressure Sensors and Artificial Intelligence Applications

As an indispensable branch of wearable electronics, flexible pressure sensors are gaining tremendous attention due to their extensive applications in health monitoring, human-machine interaction, artificial intelligence, the internet of things, and other fields. In recent years, highly flexible and wearable pressure sensors have been developed using various materials/structures and transduction mechanisms. Morphological engineering of sensing materials at the nanometer and micrometer scales is crucial to obtaining superior sensor performance. This review focuses on the rapid development of morphological engineering technologies for flexible pressure sensors. We discuss different architectures and morphological designs of sensing materials to achieve high performance, including high sensitivity, broad working range, stable sensing, low hysteresis, high transparency, and directional or selective sensing. Additionally, the general fabrication techniques are summarized, including self-assembly, patterning, and auxiliary synthesis methods. Furthermore, we present the emerging applications of high-performing microengineered pressure sensors in healthcare, smart homes, digital sports, security monitoring, and machine learning-enabled computational sensing platform. Finally, the potential challenges and prospects for the future developments of pressure sensors are discussed comprehensively.