WO3 nanorods/graphene nanocomposites for high-efficiency visible-light-driven photocatalysis and NO2 gas sensing

被引:489
|
作者
An, Xiaoqiang [1 ,2 ]
Yu, Jimmy C. [1 ,2 ]
Wang, Yu [3 ,4 ]
Hu, Yongming [3 ,4 ]
Yu, Xuelian [5 ]
Zhang, Guangjin [5 ]
机构
[1] Chinese Univ Hong Kong, Dept Chem, Shatin, Hong Kong, Peoples R China
[2] Chinese Univ Hong Kong, Inst Environm Energy & Sustainabil, Shatin, Hong Kong, Peoples R China
[3] Hong Kong Polytech Univ, Dept Appl Phys, Hong Kong, Hong Kong, Peoples R China
[4] Hong Kong Polytech Univ, Mat Res Ctr, Hong Kong, Hong Kong, Peoples R China
[5] Chinese Acad Sci, Inst Proc Engn, Beijing 100190, Peoples R China
基金
美国国家科学基金会;
关键词
REDUCED GRAPHENE OXIDE; TUNGSTEN-OXIDE; ELECTROCHROMIC PROPERTIES; HYDROGEN-PRODUCTION; CARBON NANOTUBES; NANORODS; COMPOSITES; FILMS; NANOSTRUCTURES; NANOPARTICLES;
D O I
10.1039/c2jm16709c
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
One-dimensional (1-D) nanostructures are of great importance due to their superior charge transport properties. Anchoring 1-D semiconductor nanomaterials on graphene offers potential advantages in photoelectrochemical and sensing applications. This paper presents a systematic investigation on the incorporation of WO3 nanorods and graphene for high-efficiency visible-light-driven photocatalysis and NO2 gas sensing. This novel composite shows remarkably enhanced performance compared to pure WO3 nanorods for these applications. The high photocatalytic activity of the WO3/graphene nanocomposite is found to be related to the increased adsorption toward chemical species, enhanced light absorption and efficient charge separation and transfer. Meanwhile, the improved conductivity, specific electron transfer and increased gas adsorption also contribute to their superior sensitivity and selectivity to NO2 gas.
引用
收藏
页码:8525 / 8531
页数:7
相关论文
共 50 条
  • [21] Visible-light-driven photocatalysis of heterostructure Ag/Bi2WO6 nanocomposites and their photocatalytic degradation of dye under visible light irradiation
    Phattranit Dumrongrojthanath
    Anukorn Phuruangrat
    Patcharanan Junploy
    Somchai Thongtem
    Titipun Thongtem
    Research on Chemical Intermediates, 2016, 42 : 1651 - 1662
  • [22] Visible-light-driven photocatalysis of heterostructure Ag/Bi2WO6 nanocomposites and their photocatalytic degradation of dye under visible light irradiation
    Dumrongrojthanath, Phattranit
    Phuruangrat, Anukorn
    Junploy, Patcharanan
    Thongtem, Somchai
    Thongtem, Titipun
    RESEARCH ON CHEMICAL INTERMEDIATES, 2016, 42 (03) : 1651 - 1662
  • [23] Synthesis of Fe-doped WO3 nanostructures with high visible-light-driven photocatalytic activities
    Song, Hui
    Li, Yaguang
    Lou, Zirui
    Xiao, Mu
    Hu, Liang
    Ye, Zhizhen
    Zhu, Liping
    APPLIED CATALYSIS B-ENVIRONMENTAL, 2015, 166 : 112 - 120
  • [24] Highly sensitive and rapidly responding room-temperature NO2 gas sensors based on WO3 nanorods/sulfonated graphene nanocomposites
    Wang, Tingting
    Hao, Juanyuan
    Zheng, Shengliang
    Sun, Quan
    Zhang, Di
    Wang, You
    NANO RESEARCH, 2018, 11 (02) : 791 - 803
  • [25] Hollow mesoporous TiO2/WO3 sphere heterojunction with high visible-light-driven photocatalytic activity
    Wei, Yuelin
    Huang, Yunfang
    Fang, Yu
    Zhao, Yuezhu
    Luo, Dan
    Guo, Qiyao
    Fan, Leqing
    Wu, Jihuai
    MATERIALS RESEARCH BULLETIN, 2019, 119
  • [26] Highly sensitive and rapidly responding room-temperature NO2 gas sensors based on WO3 nanorods/sulfonated graphene nanocomposites
    Tingting Wang
    Juanyuan Hao
    Shengliang Zheng
    Quan Sun
    Di Zhang
    You Wang
    Nano Research, 2018, 11 : 791 - 803
  • [27] Visible-light-driven Bi2O3/WO3 composites with enhanced photocatalytic activity
    Adhikari, Shiba P.
    Dean, Hunter
    Hood, Zachary D.
    Peng, Rui
    More, Karren L.
    Ivanov, Ilia
    Wu, Zili
    Lachgar, Abdou
    RSC ADVANCES, 2015, 5 (111): : 91094 - 91102
  • [28] Synthesis of novel AgI/BiOI nanocomposites and their high-efficiency visible-light-driven photocatalytic degradation performance for norfloxacin
    Liu, Xiaomeng
    Zhong, Yitian
    Feng, Haosheng
    Zhao, Yanxi
    Li, Qin
    Huang, Tao
    NEW JOURNAL OF CHEMISTRY, 2024, 48 (02) : 800 - 810
  • [29] Faster response of NO2 sensing in graphene-WO3 nanocomposites
    Srivastava, Shubhda
    Jain, Kiran
    Singh, V. N.
    Singh, Sukhvir
    Vijayan, N.
    Dilawar, Nita
    Gupta, Govind
    Senguttuvan, T. D.
    NANOTECHNOLOGY, 2012, 23 (20)
  • [30] Regulation of morphology and visible light-driven photocatalysis of WO3 nanostructures by changing pH
    You-Shu Fan
    Xiao-Li Xi
    Yang-Si Liu
    Zuo-Ren Nie
    Lin-Yan Zhao
    Qing-Hua Zhang
    Rare Metals, 2021, 40 : 1738 - 1745