Synthesis and Characterization of Solution-Processable Ladderized n-Type Naphthalene Bisimide Copolymers for OFET Applications

被引：98
|
作者：
Durban, Matthew M. [2 ]
Kazarinoff, Peter D. [1 ]
Segawa, Yukari [1 ,3 ]
Luscombe, Christine K. [1 ]
机构：
[1] Univ Washington, Dept Mat Sci & Engn, Seattle, WA 98195 USA
[2] Univ Washington, Dept Chem, Seattle, WA 98195 USA
[3] Tokyo Inst Technol, Grad Sch Engn, Dept Organ & Polymer Mat, Meguro Ku, Tokyo 1528552, Japan
来源：
MACROMOLECULES | 2011年 / 44卷 / 12期
基金：
美国国家科学基金会;
关键词：
THIN-FILM TRANSISTORS; INTRAMOLECULAR CHARGE-TRANSFER; FIELD-EFFECT TRANSISTORS; HIGH-ELECTRON-MOBILITY; DIIMIDE SEMICONDUCTORS; ORGANIC SEMICONDUCTORS; HIGH-PERFORMANCE; PI-CONJUGATION; POLYMERS; PLANAR;
D O I：
10.1021/ma2004822
中图分类号：
O63 [高分子化学（高聚物）];
学科分类号：
070305 ; 080501 ; 081704 ;
摘要：
Solution-processable n-type ladder-based polymers are highly desirable due to their potential capability to form strong. pi-pi interactions. A series of 5 highly soluble naphthalene diimide (NDI) polymers are presented, differing in the degree to which they are able to form imine-bridged ladder polymer structures. Average electron mobilities as high as 0.0026 cm(2) V-1 s(-1), which show an electron-mobility improvement of 4 orders of magnitude following ladderization, and on/off current ratios on the order of 10(4) are reported for the novel material PNDI-2BocL, an alkyl-substituted poly(benzoquinolinophenanthrolinedione). The structure property relationship of the aforementioned series of copolymers is presented and discussed as it pertains to organic field-effect transistor (OFET) performance.
引用
收藏
页码：4721 / 4728
页数：8
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