Sulfur conversions during coal char gasification with a two-stage air supply in a pilot-scale circulating fluidized bed gasifier

被引：6
|
作者：
Chai, Zhen [1 ]
Zhu, Zhiping [2 ]
Wang, Xiaofang [1 ]
Wang, Kun [1 ]
机构：
[1] Chinese Acad Sci, Inst Engn Thermophys, Beijing, Peoples R China
[2] Chinese Acad Sci, Inst Engn Thermophys, Univ Chinese Acad Sci, Beijing, Peoples R China
来源：
ENERGY SOURCES PART A-RECOVERY UTILIZATION AND ENVIRONMENTAL EFFECTS | 2020年 / 42卷 / 04期
关键词：
Coal char; gasification; sulfur conversion; circulating fluidized bed gasifier; two-stage air supply; BIOMASS GASIFICATION; PARTICLE-SIZE; TRANSFORMATION; PYROLYSIS; GAS; COMBUSTION; REMOVAL; LIGNITE; PYRITE; NH3;
D O I：
10.1080/15567036.2019.1587088
中图分类号：
TE [石油、天然气工业]; TK [能源与动力工程];
学科分类号：
0807 ; 0820 ;
摘要：
This paper aims at studying sulfur conversions in a pilot-scale circulating fluidized bed (CFB) gasification system of two-stage air supply. The effects of different air supply approaches, secondary air supply heights and gasification agent compositions on gasifier temperature, sulfur conversions and the release of hydrogen sulfide (H2S) and carbonyl sulfide (COS) were investigated. Two-stage air supply approaches optimized CFB gasifier temperature profile and enhanced sulfur conversions to gas. Sulfur conversions to gas decreased with the increase of secondary air supply nozzle location height. The increased steam-to-carbon ratio promoted sulfur release, leading to more H2S and less COS release.
引用
收藏
页码：421 / 431
页数：11
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