Sulfur conversions during coal char gasification with a two-stage air supply in a pilot-scale circulating fluidized bed gasifier

被引:6
|
作者
Chai, Zhen [1 ]
Zhu, Zhiping [2 ]
Wang, Xiaofang [1 ]
Wang, Kun [1 ]
机构
[1] Chinese Acad Sci, Inst Engn Thermophys, Beijing, Peoples R China
[2] Chinese Acad Sci, Inst Engn Thermophys, Univ Chinese Acad Sci, Beijing, Peoples R China
关键词
Coal char; gasification; sulfur conversion; circulating fluidized bed gasifier; two-stage air supply; BIOMASS GASIFICATION; PARTICLE-SIZE; TRANSFORMATION; PYROLYSIS; GAS; COMBUSTION; REMOVAL; LIGNITE; PYRITE; NH3;
D O I
10.1080/15567036.2019.1587088
中图分类号
TE [石油、天然气工业]; TK [能源与动力工程];
学科分类号
0807 ; 0820 ;
摘要
This paper aims at studying sulfur conversions in a pilot-scale circulating fluidized bed (CFB) gasification system of two-stage air supply. The effects of different air supply approaches, secondary air supply heights and gasification agent compositions on gasifier temperature, sulfur conversions and the release of hydrogen sulfide (H2S) and carbonyl sulfide (COS) were investigated. Two-stage air supply approaches optimized CFB gasifier temperature profile and enhanced sulfur conversions to gas. Sulfur conversions to gas decreased with the increase of secondary air supply nozzle location height. The increased steam-to-carbon ratio promoted sulfur release, leading to more H2S and less COS release.
引用
收藏
页码:421 / 431
页数:11
相关论文
共 50 条
  • [1] Pilot verification of a low-tar two-stage coal gasification process with a fluidized bed pyrolyzer and fixed bed gasifier
    Zeng, Xi
    Wang, Fang
    Li, Hongling
    Wang, Yin
    Dong, Li
    Yu, Jian
    Xu, Guangwen
    APPLIED ENERGY, 2014, 115 : 9 - 16
  • [2] Radiotracer investigation in a pilot-scale fluidized bed coal gasifier (FBCG)
    Goswami, Sunil
    Pant, H. J.
    Sharma, V. K.
    Varshney, Lalit
    APPLIED RADIATION AND ISOTOPES, 2019, 149 : 22 - 30
  • [3] Enhancement of coal char gasification using a pyrolyzer-gasifier isolated circulating fluidized bed gasification system
    Matsuoka, Koichi
    Hosokai, Sou
    Kuramoto, Koji
    Suzuki, Yoshizo
    FUEL PROCESSING TECHNOLOGY, 2013, 109 : 43 - 48
  • [4] Study on the gasification of pine sawdust with dolomite catalyst in a pilot-scale fluidized bed gasifier
    Wang, Duo
    Liu, Yun-Quan
    Li, Wen-Ping
    Wei, Mi-Mi
    Ye, Yue-Yuan
    Li, Shui-Rong
    Wang, Meng
    ENERGY SOURCES PART A-RECOVERY UTILIZATION AND ENVIRONMENTAL EFFECTS, 2019, 42 (09) : 1132 - 1139
  • [5] Gasification of biomass with oxygen-enriched air in a pilot scale two-stage gasifier
    Wang, Zhiqi
    He, Tao
    Qin, Jianguang
    Wu, Jingli
    Li, Jianqing
    Zi, Zhongyue
    Liu, Guangbo
    Wu, Jinhu
    Sun, Li
    FUEL, 2015, 150 : 386 - 393
  • [6] Co-gasification of high ash Indian coal-biomass blends in a pilot-scale fluidized bed gasifier
    Datta, Sudipta
    Chauhan, Vishal
    Sahu, Gajanan
    Chavan, Prakash D.
    Saha, Sujan
    Gupta, Pavan K.
    Dutta, Pashupati
    BIOMASS CONVERSION AND BIOREFINERY, 2020, 10 (04) : 831 - 838
  • [7] Co-gasification of high ash Indian coal-biomass blends in a pilot-scale fluidized bed gasifier
    Sudipta Datta
    Vishal Chauhan
    Gajanan Sahu
    Prakash D. Chavan
    Sujan Saha
    Pavan K. Gupta
    Pashupati Dutta
    Biomass Conversion and Biorefinery, 2020, 10 : 831 - 838
  • [8] CFD modeling for coal size effect on coal gasification in a two-stage commercial entrained-bed gasifier with an improved char gasification model
    Jeong, Hyo Jae
    Seo, Dong Kyun
    Hwang, Jungho
    APPLIED ENERGY, 2014, 123 : 29 - 36
  • [9] MODELING A PILOT-SCALE FLUIDIZED-BED COAL-GASIFICATION REACTOR
    MA, RP
    FELDER, RM
    FERRELL, JK
    FUEL PROCESSING TECHNOLOGY, 1988, 19 (03) : 265 - 290
  • [10] Parametric and hydrodynamics studies on gasification performance of biomass pellets in a pilot-scale fluidized bed gasifier
    Emiola-Sadiq, Tolu
    Zhang, Lifeng
    Dalai, Ajay
    Gerspacher, Regan
    Campbell, Bill
    Evitts, Richard
    BIOMASS CONVERSION AND BIOREFINERY, 2024, 14 (14) : 16339 - 16361