Large-scale, low-cost, broadband and tunable perfect optical absorber based on phase-change material

被引:119
|
作者
Mou, Nanli [1 ,2 ]
Liu, Xiaolong [3 ,4 ]
Wei, Tao [1 ]
Dong, Hongxing [1 ]
He, Qiong [5 ,6 ,7 ]
Zhou, Lei [5 ,6 ,7 ]
Zhang, Yaqiang [1 ,2 ]
Zhang, Long [1 ]
Sun, Shulin [3 ,4 ]
机构
[1] Chinese Acad Sci, Shanghai Inst Opt & Fine Mech, Key Lab Mat High Power Laser, Shanghai 201800, Peoples R China
[2] Univ Chinese Acad Sci, Ctr Mat Sci & Optoelect Engn, Beijing 100049, Peoples R China
[3] Fudan Univ, Shanghai Engn Res Ctr Ultra Precis Opt Mfg, Green Photon, Shanghai 200433, Peoples R China
[4] Fudan Univ, Dept Opt Sci & Engn, Shanghai 200433, Peoples R China
[5] Fudan Univ, State Key Lab Surface Phys, Shanghai 200433, Peoples R China
[6] Fudan Univ, Key Lab Micro & Nano Photon Struct, Minist Educ, Shanghai 200433, Peoples R China
[7] Collaborat Innovat Ctr Adv Microstruct, Nanjing 210093, Peoples R China
基金
中国国家自然科学基金;
关键词
METAMATERIAL ABSORBERS; ABSORPTION; ULTRABROADBAND; HYBRIDIZATION; LIGHT;
D O I
10.1039/c9nr07602f
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Metamaterial-based electromagnetic absorbers have attracted much attention recently, but most previous realizations suffer from issues of narrow bandwidth, time-consuming and high-cost fabrication methods, and/or fixed functionalities, and so are unfavorable for practical applications. Here, we demonstrate experimentally a large-scale, broadband, polarization-independent, and tunable metamaterial absorber, which works for both visible and near-infrared light. A lithography-free and low-cost method was utilized to fabricate a centimeter-sized metamaterial sample in a metal-insulator-metal (MIM) configuration with nano-scale precision, in which a phase-change material, Ge2Sb2Te5 (GST), was adopted as the insulating spacer of the MIM structure. With two different resonance mechanisms working together, the proposed device was shown to exhibit high absorptivity (>80%) within a broad wavelength band (480-1020 nm). By thermally tuning the phase state of the GST layer, we can dramatically enlarge the working bandwidth of the metamaterial absorber by shifting one absorption peak by about 470 nm. These findings may stimulate many potential applications in, for example, solar cells, energy harvesting, smart sensing/imaging, and color printing.
引用
收藏
页码:5374 / 5379
页数:6
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