Source apportionment and seasonal variation of PM2.5 carbonaceous aerosol in the Beijing-Tianjin-Hebei Region of China

被引:110
|
作者
Wang, Gang [1 ,3 ]
Cheng, Shuiyuan [1 ,3 ]
Li, Jianbing [2 ]
Lang, Jianlei [1 ,3 ]
Wen, Wei [1 ,3 ]
Yang, Xiaowen [1 ,3 ]
Tian, Liang [1 ,3 ]
机构
[1] Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Beijing 100022, Peoples R China
[2] Univ No British Columbia, Environm Engn Program, Prince George, BC V2N 4Z9, Canada
[3] Collaborat Innovat Ctr Elect Vehicles, Beijing 100081, Peoples R China
关键词
Carbonaceous aerosol; Elemental carbon; Organic carbon; PM2.5; Principal component analysis; SECONDARY ORGANIC AEROSOL; ELEMENTAL CARBON; CHEMICAL-COMPOSITION; DESCRIPTIVE ANALYSIS; SOURCE PROFILES; HONG-KONG; URBAN; TEMPERATURE; VISIBILITY; EMISSIONS;
D O I
10.1007/s10661-015-4288-x
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
The seasonal variation of PM2.5 carbonaceous aerosol was investigated in Beijing and Tangshan cities of China. The characteristics of carbonaceous aerosol (e.g., organic carbon, OC and elemental carbon, EC) under different weather conditions and their source apportionment were also examined. The annual average PM2.5 concentration in the study area reached 95.6-197.3 mu g/m(3), showing seasonal and spatial variation. The carbonaceous materials accounted for 17.3-21.2% of the PM2.5, and they had a much higher content under haze weather condition. It was found that the PM2.5 contained more OC than EC. Principal component analysis (PCA) results indicated that the carbonaceous components came from mixed emission sources of coal combustion, vehicle exhaust, and biomass burning. In Beijing, the vehicle emission made a contribution of 63.0 % to the carbonaceous components of PM2.5 in summer, which is higher than that in Tangshan. While in Tangshan, the coal combustion made a contribution of 30.3 %, which is much higher than that in Beijing.
引用
收藏
页数:13
相关论文
共 50 条
  • [31] Pollution characteristic of PM2.5 and secondary inorganic ions in Beijing-Tianjin-Hebei region.
    Jia, Jia
    Han, Li-Hui
    Cheng, Shui-Yuan
    Zhang, Han-Yu
    Lv, Zhe
    Zhongguo Huanjing Kexue/China Environmental Science, 2018, 38 (03): : 801 - 811
  • [32] Can MODIS AOD be employed to derive PM2.5 in Beijing-Tianjin-Hebei over China?
    Ma, Xiaoyan
    Wang, Jianying
    Yu, Fangqun
    Jia, Hailing
    Hu, Yanan
    ATMOSPHERIC RESEARCH, 2016, 181 : 250 - 256
  • [33] Optimization of Seasonal Geographically and Temporally Weighted Regression Model for Accurate Estimation of Seasonal PM2.5 Concentrations in Beijing-Tianjin-Hebei Region
    Zhou, Lei
    Wang, Yani
    Du, Mingyi
    Jing, Changfeng
    Wang, Siyu
    Zhu, Yinuo
    Luo, Ting
    He, Congcong
    Gao, Ting
    Yang, Kun
    SENSORS AND MATERIALS, 2020, 32 (12) : 4393 - 4412
  • [34] Source apportionment of PM2.5 carbonaceous aerosol in Baghdad, Iraq
    Hamad, Samera Hussein
    Schauer, James Jay
    Heo, Jongbae
    Kadhim, Ahmed K. H.
    ATMOSPHERIC RESEARCH, 2015, 156 : 80 - 90
  • [35] Characteristics of concentrations and chemical compositions for PM2.5 in the region of Beijing, Tianjin, and Hebei, China
    Zhao, P. S.
    Dong, F.
    He, D.
    Zhao, X. J.
    Zhang, X. L.
    Zhang, W. Z.
    Yao, Q.
    Liu, H. Y.
    ATMOSPHERIC CHEMISTRY AND PHYSICS, 2013, 13 (09) : 4631 - 4644
  • [36] Retrieval of Daily PM2.5 Concentrations Using Nonlinear Methods: A Case Study of the Beijing-Tianjin-Hebei Region, China
    Li, Lijuan
    Chen, Baozhang
    Zhang, Yanhu
    Zhao, Youzheng
    Xian, Yue
    Xu, Guang
    Zhang, Huifang
    Guo, Lifeng
    REMOTE SENSING, 2018, 10 (12)
  • [37] The contribution of residential coal combustion to PM2.5 pollution over China's Beijing-Tianjin-Hebei region in winter
    Zhang, Zhongzhi
    Wang, Wenxing
    Cheng, Miaomiao
    Liu, Shijie
    Xu, Jun
    He, Youjiang
    Meng, Fan
    ATMOSPHERIC ENVIRONMENT, 2017, 159 : 147 - 161
  • [38] Hazard posed by metals and As in PM2.5 in air of five megacities in the Beijing-Tianjin-Hebei region of China during APEC
    Zhang, Linlin
    Jin, Xiaowei
    Johnson, Andrew C.
    Giesy, John P.
    ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH, 2016, 23 (17) : 17603 - 17612
  • [39] Hazard posed by metals and As in PM2.5 in air of five megacities in the Beijing-Tianjin-Hebei region of China during APEC
    Linlin Zhang
    Xiaowei Jin
    Andrew C. Johnson
    John P. Giesy
    Environmental Science and Pollution Research, 2016, 23 : 17603 - 17612
  • [40] The environmental Kuznets curve for PM2.5 pollution in Beijing-Tianjin-Hebei region of China: A spatial panel data approach
    Ding, Yueting
    Zhang, Ming
    Chen, Sai
    Wang, Wenwen
    Nie, Rui
    JOURNAL OF CLEANER PRODUCTION, 2019, 220 : 984 - 994