Solid state 31P and 207Pb MAS NMR studies on polycrystalline 0,0′-dialkyldithiophosphate lead(II) complexes

被引：35

作者：

Larsson, AC

Ivanov, AV

Pike, KJ

Forsling, W

Antzutkin, ON ^{[1
]}

机构：

[1] Univ Lulea, Div Chem, S-97187 Lulea, Sweden

[2] Russian Acad Sci, Far Eastern Branch, Amur Integrated Res Inst, Blagoveshchensk 675000, Russia

[3] ANSTO, Mat & Engn Sci, Lucas Heights, NSW 2234, Australia

来源：

JOURNAL OF MAGNETIC RESONANCE | 2005年 / 177卷 / 01期

关键词：

P-31; CP/MAS; (207) Pb MAS NMR; P-31 chemical shift anisotropy; (207) Pb chemical shift anisotropy; 0,0 '-dialkyldithiophosphate lead(II) complexes; (2)J(P-31; (207); Pb)-coupling;

D O I：

10.1016/j.jmr.2005.07.007

中图分类号：

Q5 [生物化学];

学科分类号：

071010 ; 081704 ;

摘要：

A number of lead(II) O,O'-dialkyldithiophosphate complexes were studied by C-13, P-31, and Pb-207 MAS NMR. Simulations of P-31 chemical shift anisotropy using spinning sideband analysis reveal a linear relationship between the S-P-S bond angle and the principal values delta(22) and delta(33) of the P-31 chemical shift tensor. The P-31 CSA data were used to assign ligands with different structural functions. In the cases of diethyldithiophosphate and di-iso-butyldithiophosphate lead(II) complexes, (2)J(P-31, Pb-207)-couplings were resolved and used to confirm the suggested assignment of the ligands. The SIMPSON computer program was used to calculate P-31 and Pb-207 spectral sideband patterns. (c) 2005 Elsevier Inc. All rights reserved.

引用

页码：56 / 66

页数：11

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